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Singlet Oxygen Generation by Novel NIR BODIPY Dyes
Abstract
Five novel near-infrared BODIPY dyes were prepared for improved singlet oxygen generation using thiophene and bromine. Theoretical, optical, photostable, and singlet oxygen generation characteristics of these dyes were assessed. Predicted excitation energies by TDDFT calculations were in good agreement (ΔE ≈ 0.06 eV) with experimental data. All five dyes showed both excitation and emission in the NIR range. In particular, two dyes having sulfur and bromine atoms showed efficient singlet oxygen generation with high photostability.
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Cites
BODIPY Dyes and Their Derivatives: Syntheses and Spectroscopic Properties
Loudet, A., & Burgess, K. (2007) · Chemical Reviews · doi:10.1021/cr078381n · Cited by 5,238
Definition of type I and type II photosensitized oxidation
Foote, C. S. (1991) · Photochemistry and Photobiology · doi:10.1111/j.1751-1097.1991.tb02071.x · Cited by 1,248
Cited by
Recent Strategies to Develop Innovative Photosensitizers for Enhanced Photodynamic Therapy
Pham, T. C., Nguyen, V.-N., Choi, Y., Lee, S., & Yoon, J. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00381 · Cited by 1,813
Triplet photosensitizers: from molecular design to applications
Zhao, J., Wu, W., Sun, J., & Guo, S. (2013) · Chemical Society Reviews · doi:10.1039/c3cs35531d · Cited by 1,579
Photosensitizers with Aggregation‐Induced Emission: Materials and Biomedical Applications
Hu, F., Xu, S., & Liu, B. (2018) · Advanced Materials · doi:10.1002/adma.201801350 · Cited by 859
Dye chemistry with time-dependent density functional theory
Laurent, A. D., Adamo, C., & Jacquemin, D. (2014) · Phys. Chem. Chem. Phys. · doi:10.1039/c3cp55336a · Cited by 398
Metadata
- Authors
- Awuah, S. G., Polreis, J., Biradar, V., & You, Y.
- Venue
- Organic Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-07-06
- Volume
- 13
- Issue
- 15
- Pages
- 3884-3887
- ISSN
- 1523-7052 (ISSN-L)
- 1523-7060
- OpenAlex
- W2314990448
- Cited by
- 237
- References
- 2
- FWCI
- 8.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Awuah, S. G., Polreis, J., Biradar, V., & You, Y. (2011). Singlet Oxygen Generation by Novel NIR BODIPY Dyes. Organic Letters. https://doi.org/10.1021/ol2014076
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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