The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
A large organic aerosol source in the free troposphere missing from current models
Open accessAbstract
Aircraft measurements of organic carbon (OC) aerosol by two independent methods over the NW Pacific during the ACE‐Asia campaign reveal unexpectedly high concentrations in the free troposphere (FT). Concentrations average 4 μg sm−3 in the 2–6.5 km column with little vertical gradient. These values are 10–100 times higher than computed with a global chemical transport model (CTM) including a standard 2‐product simulation of secondary organic aerosol (SOA) formation based on empirical fits to smog chamber data. The same CTM reproduces the observed vertical profiles of sulfate and elemental carbon aerosols, which indicate sharp decreases from the boundary layer to the FT due to wet scavenging. Our results suggest a large, sustained source of SOA in the FT from oxidation of long‐lived volatile organic compounds. We find that this SOA is the dominant component of aerosol mass in the FT, with implications for intercontinental pollution transport and radiative forcing of climate.
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Murphy, D. M., Thomson, D. S., & Mahoney, M. J. (1998) · Science · doi:10.1126/science.282.5394.1664 · Cited by 571
Cited by
Evolution of Organic Aerosols in the Atmosphere
Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., et al. (2009) · Science · doi:10.1126/science.1180353 · Cited by 4,167
van Donkelaar, A., Martin, R. V., Brauer, M., Kahn, R., Levy, R., Verduzco, C., & Villeneuve, P. J. (2010) · Environmental Health Perspectives · doi:10.1289/ehp.0901623 · Cited by 1,623
Formation of Urban Fine Particulate Matter
Zhang, R., Wang, G., Guo, S., Zamora, M. L., Ying, Q., Lin, Y., Wang, W., Hu, M., & Wang, Y. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00067 · Cited by 1,426
Reactive intermediates revealed in secondary organic aerosol formation from isoprene
Surratt, J. D., Chan, A. W. H., Eddingsaas, N. C., Chan, M., Loza, C. L., Kwan, A. J., Hersey, S. P., Flagan, R. C., Wennberg, P. O., & Seinfeld, J. H. (2010) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0911114107 · Cited by 1,081
Self-citationA review of Secondary Organic Aerosol (SOA) formation from isoprene
Carlton, A. G., Wiedinmyer, C., & Kroll, J. H. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-4987-2009 · Cited by 912
Metadata
- Authors
- Heald, C. L., Jacob, D. J., Park, R. J., Russell, L. M., Huebert, B. J., Seinfeld, J. H., Liao, H., & Weber, R. J.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 2005-09-27
- Volume
- 32
- Issue
- 18
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2161164864
- Cited by
- 584
- References
- 1
- FWCI
- 22.81
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Heald, C. L., Jacob, D. J., Park, R. J., Russell, L. M., Huebert, B. J., Seinfeld, J. H., Liao, H., & Weber, R. J. (2005). A large organic aerosol source in the free troposphere missing from current models. Geophysical Research Letters. https://doi.org/10.1029/2005gl023831
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