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Balloonborne measurements of the Pinatubo aerosol size distribution and volatility at Laramie, Wyoming during the summer of 1991
Abstract
Measurements using balloonborne optical particle counters at Laramie, Wyoming during the summer of 1991 are used to study the particle size distribution and volatility of the aerosol which formed in the stratosphere following the mid‐June eruptions of Mt. Pinatubo. Enhanced aerosol layers were observed below 20 km as early as 16 July, about 1 month after the eruption. During late July, a transient though substantial particle layer was observed in the 23 km region. High concentrations of large particles in this high altitude layer resulted in aerosol mass mixing ratios as large as 0.5 ppm, considerably larger than observed following the eruption of El Chichón. Aerosol volatility tests indicated that well over 90% of the particles were composed of an H 2 SO 4/H 2 O solution in all layers observed, indicating rapid conversion of SO 2 to H 2 SO 4 and subsequent droplet growth. High concentrations of droplets suggest homogeneous or ion nucleation as the most likely aerosol production mechanism.
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Citations
Cited by
Vehkamäki, H., Kulmala, M., Napari, I., Lehtinen, K. E. J., Timmreck, C., Noppel, M., & Laaksonen, A. (2002) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2002jd002184 · Cited by 663
Global direct radiative forcing due to multicomponent anthropogenic and natural aerosols
Jacobson, M. Z. (2001) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2000jd900514 · Cited by 462
Radiative Climate Forcing by the Mount Pinatubo Eruption
Minnis, P., Harrison, E. F., Stowe, L. L., Gibson, G. G., Denn, F. M., Doelling, D. R., & Smith, W. L. (1993) · Science · doi:10.1126/science.259.5100.1411 · Cited by 374
Carslaw, K. S., Luo, B. P., Clegg, S. L., Peter, T., Brimblecombe, P., & Crutzen, P. J. (1994) · Geophysical Research Letters · doi:10.1029/94gl02799 · Cited by 374
The impact of geoengineering aerosols on stratospheric temperature and ozone
Heckendorn, P., Weisenstein, D., Fueglistaler, S., Luo, B. P., Rozanov, E., Schraner, M., Thomason, L. W., & Peter, T. (2009) · Environmental Research Letters · doi:10.1088/1748-9326/4/4/045108 · Cited by 254
Metadata
- Authors
- Deshler, T., Hofmann, D. J., Johnson, B. J., & Rozier, W. R.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 1992-01-24
- Volume
- 19
- Issue
- 2
- Pages
- 199-202
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2104953453
- Cited by
- 188
- References
- 0
- FWCI
- 38.18
- Type
- journal article
- Language
- en
- Open access
- closed
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- Deshler, T., Hofmann, D. J., Johnson, B. J., & Rozier, W. R. (1992). Balloonborne measurements of the Pinatubo aerosol size distribution and volatility at Laramie, Wyoming during the summer of 1991. Geophysical Research Letters. https://doi.org/10.1029/91gl02787
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.