The DOI matches its Crossref record; 17 of the 17 references it cites were found in a registry or an index.
Stratospheric aerosol growth and HNO3 gas phase depletion from coupled HNO3 and water uptake by liquid particles
Abstract
Aqueous sulphuric acid droplets, which constitute the background stratospheric aerosol, strongly absorb HNO 3 and HCl under cold conditions. A thermodynamic model is used to predict partitioning of HNO 3, HCl and H 2 O between gas and aerosol phases, and show that a 50‐fold increase in aerosol volume, observed in the Arctic stratosphere as temperature approached the frost point (188.9 K), can be explained in terms of uptake of HNO 3 and H 2 O by liquid aerosols. Calculated degrees of saturation of the droplets with respect to solid hydrates, taking into account the reduction in vapour phase HNO 3, suggest that the droplets remain liquid to the frost point. Near this temperature, they can yield larger aerosol volumes than would have been the case for solid NAT (HNO 3•3H 2 O) particles. The depletion of gas phase HNO 3 into enhanced volumes of liquid aerosols resulting from volcanic eruptions may hamper NAT formation.
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Cites
Laboratory studies of the nitric acid trihydrate: Implications for the south polar stratosphere
Hanson, D., & Mauersberger, K. (1988) · Geophysical Research Letters · doi:10.1029/gl015i008p00855 · Cited by 755
Heterogeneous reactions in sulfuric acid aerosols: A framework for model calculations
Hanson, D. R., Ravishankara, A. R., & Solomon, S. (1994) · Journal of Geophysical Research: Atmospheres · doi:10.1029/93jd02932 · Cited by 473
Clegg, S. L., Pitzer, K. S., & Brimblecombe, P. (1992) · The Journal of Physical Chemistry · doi:10.1021/j100202a074 · Cited by 362
Self-citationDye, J. E., Baumgardner, D., Gandrud, B. W., Kawa, S. R., Kelly, K. K., Loewenstein, M., Ferry, G. V., Chan, K. R., & Gary, B. L. (1992) · Journal of Geophysical Research: Atmospheres · doi:10.1029/91jd02740 · Cited by 259
Physical Chemistry of the H 2 SO 4 /HNO 3 /H 2 O System: Implications for Polar Stratospheric Clouds
Molina, M. J., Zhang, R., Wooldridge, P. J., McMahon, J. R., Kim, J. E., Chang, H. Y., & Beyer, K. D. (1993) · Science · doi:10.1126/science.261.5127.1418 · Cited by 257
Role of heterogeneous conversion of N2O5 on sulphate aerosols in global ozone losses
Rodriguez, J. M., Ko, M. K. W., & Sze, N. D. (1991) · Nature · doi:10.1038/352134a0 · Cited by 231
A study of type I polar stratospheric cloud formation
Tabazadeh, A., Turco, R. P., Drdla, K., Jacobson, M. Z., & Toon, O. B. (1994) · Geophysical Research Letters · doi:10.1029/94gl01368 · Cited by 223
An analysis of lidar observations of polar stratospheric clouds
Toon, O. B., Browell, E. V., Kinne, S., & Jordan, J. (1990) · Geophysical Research Letters · doi:10.1029/gl017i004p00393 · Cited by 193
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A model for studying the composition and chemical effects of stratospheric aerosols
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Cited by
Stratospheric ozone depletion: A review of concepts and history
Solomon, S. (1999) · Reviews of Geophysics · doi:10.1029/1999rg900008 · Cited by 2,008
Thermodynamic Model of the System H+−NH4+−SO42-−NO3-−H2O at Tropospheric Temperatures
Clegg, S. L., Brimblecombe, P., & Wexler, A. S. (1998) · The Journal of Physical Chemistry A · doi:10.1021/jp973042r · Cited by 782
Self-citationPhase Transitions of Aqueous Atmospheric Particles
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Voigt, C., Schlager, H., Luo, B. P., Dörnbrack, A., Roiger, A., Stock, P., Curtius, J., Vössing, H., Borrmann, S., Davies, S., et al. (2005) · Atmospheric Chemistry and Physics · doi:10.5194/acp-5-1371-2005 · Cited by 161
Self-citationObservations of the chemical composition of stratospheric aerosol particles
Murphy, D. M., Froyd, K. D., Schwarz, J. P., & Wilson, J. C. (2014) · Quarterly Journal of the Royal Meteorological Society · doi:10.1002/qj.2213 · Cited by 141
Metadata
- Authors
- Carslaw, K. S., Luo, B. P., Clegg, S. L., Peter, T., Brimblecombe, P., & Crutzen, P. J.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 1994-11-15
- Volume
- 21
- Issue
- 23
- Pages
- 2479-2482
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2030397317
- Cited by
- 374
- References
- 17
- FWCI
- 25.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Carslaw, K. S., Luo, B. P., Clegg, S. L., Peter, T., Brimblecombe, P., & Crutzen, P. J. (1994). Stratospheric aerosol growth and HNO3 gas phase depletion from coupled HNO3 and water uptake by liquid particles. Geophysical Research Letters. https://doi.org/10.1029/94gl02799
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
