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Chemistry of the 1991–1992 stratospheric winter: Three‐dimensional model simulations
Open accessAbstract
A three‐dimensional chemistry‐transport model of the stratosphere is used to simulate the evolution of trace constituents during the 1991–1992 Arctic winter. It is shown that heterogeneous reactions on polar stratospheric clouds led in early January to almost complete activation of atmospheric chlorine inside the polar vortex, in remarkable coincidence with observations by the ER‐2 aircraft (Toohey et al., 1993) and the microwave limb sounder on the Upper Atmosphere Research Satellite (Waters et al., 1993). Sulfate aerosols resulting from the eruption of Mount Pinatubo also produced a significant increase in chlorine monoxide (ClO) concentrations at middle and high latitudes. The net chemical destruction of ozone found in the vortex at the end of the simulation (25% at 50 hPa and 25 DU), although substantial, was limited by available sunlight and the short period during which stratospheric clouds occurred.
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Cited by
Kinnison, D. E., Brasseur, G. P., Walters, S., Garcia, R. R., Marsh, D. R., Sassi, F., Harvey, V. L., Randall, C. E., Emmons, L., Lamarque, J. F., et al. (2007) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2006jd007879 · Cited by 489
Self-citationEyring, V., Butchart, N., Waugh, D. W., Akiyoshi, H., Austin, J., Bekki, S., Bodeker, G. E., Boville, B. A., Brühl, C., Chipperfield, M. P., et al. (2006) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2006jd007327 · Cited by 429
Schmidt, H., Brasseur, G. P., Charron, M., Manzini, E., Giorgetta, M. A., Diehl, T., Fomichev, V. I., Kinnison, D., Marsh, D., & Walters, S. (2006) · Journal of Climate · doi:10.1175/jcli3829.1 · Cited by 275
Multiple symptoms of total ozone recovery inside the Antarctic vortex during austral spring
Pazmiño, A., Godin-Beekmann, S., Hauchecorne, A., Claud, C., Khaykin, S., Goutail, F., Wolfram, E., Salvador, J., & Quel, E. (2018) · Atmospheric Chemistry and Physics · doi:10.5194/acp-18-7557-2018 · Cited by 64
Hodnebrog, Ø., Berntsen, T. K., Dessens, O., Gauss, M., Grewe, V., Isaksen, I. S. A., Koffi, B., Myhre, G., Olivié, D., Prather, M. J., et al. (2011) · Atmospheric chemistry and physics · doi:10.5194/acp-11-11293-2011 · Cited by 36
Metadata
- Venue
- Journal of Geophysical Research: Atmospheres
- Publisher
- American Geophysical Union (AGU)
- Published
- 1994-04-20
- Volume
- 99
- Issue
- D4
- Pages
- 8183-8195
- ISSN
- 0148-0227 (ISSN-L)
- OpenAlex
- W1975290697
- Cited by
- 320
- References
- 0
- FWCI
- 10.27
- Type
- journal article
- Language
- en
- Open access
- green
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- Chemistry of the 1991–1992 stratospheric winter: Three‐dimensional model simulations. (1994). Journal of Geophysical Research: Atmospheres. https://doi.org/10.1029/93jd03476
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
