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Mass accommodation coefficient for HO2 radicals on aqueous particles
Abstract
The rate of reaction of gas phase HO 2 radicals with a monodisperse, submicrometer aerosol was measured in a flow tube reactor at atmospheric pressure. At the relative humidity of the experiments (75%), the aerosol consisted of concentrated solution droplets of either LiNO 3 or NH 4 HSO 4. When the aerosol contained a sufficient amount of Cu(II) ions, reaction of HO 2 with the aerosol was observed. The mass accommodation coefficient for HO 2 on aqueous particles was determined to be greater than 0.2. This implies that in clouds HO 2 mass transport will be limited by gas‐phase diffusion and HO 2 will be in equilibrium at the gas‐liquid interface. Reactions of HO 2 with Cu(I) and Cu(II) ions in submicrometer aerosols may have a significant role in converting atmospheric odd hydrogen radicals into H 2 O 2.
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Citations
Cites
Reactivity of HO2/O− 2 radicals in aqueous solution
Bielski, B. H. J., Cabelli, D. E., Arudi, R. L., & Ross, A. B. (1985) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555739 · Cited by 2,169
Cited by
Heterogeneous chemistry and tropospheric ozone
Jacob, D. (2000) · Atmospheric Environment · doi:10.1016/s1352-2310(99)00462-8 · Cited by 1,289
Atmospheric composition change – global and regional air quality
Monks, P. S., Granier, C., Fuzzi, S., Stohl, A., Williams, M. L., Akimoto, H., Amann, M., Baklanov, A., Baltensperger, U., Bey, I., et al. (2009) · Atmospheric Environment · doi:10.1016/j.atmosenv.2009.08.021 · Cited by 872
An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds
Kolb, C. E., Cox, R. A., Abbatt, J. P. D., Ammann, M., Davis, E. J., Donaldson, D. J., Garrett, B. C., George, C., Griffiths, P. T., Hanson, D. R., et al. (2010) · Atmospheric Chemistry and Physics · doi:10.5194/acp-10-10561-2010 · Cited by 405
Mass Accommodation and Chemical Reactions at Gas−Liquid Interfaces
Davidovits, P., Kolb, C. E., Williams, L. R., Jayne, J. T., & Worsnop, D. R. (2006) · Chemical Reviews · doi:10.1021/cr040366k · Cited by 306
Metadata
- Authors
- Mozurkewich, M., McMurry, P. H., Gupta, A., & Calvert, J. G.
- Venue
- Journal of Geophysical Research: Atmospheres
- Publisher
- American Geophysical Union (AGU)
- Published
- 1987-04-20
- Volume
- 92
- Issue
- D4
- Pages
- 4163-4170
- ISSN
- 0148-0227 (ISSN-L)
- OpenAlex
- W2166668914
- Cited by
- 187
- References
- 1
- FWCI
- 5.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Mozurkewich, M., McMurry, P. H., Gupta, A., & Calvert, J. G. (1987). Mass accommodation coefficient for HO2 radicals on aqueous particles. Journal of Geophysical Research: Atmospheres. https://doi.org/10.1029/jd092id04p04163
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
