The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Suppressing photochemical reactions with quantized light fields
Open accessAbstract
Photoisomerization, that is, a photochemical reaction leading to a change of molecular structure after absorption of a photon, can have detrimental effects such as leading to DNA damage under solar irradiation, or as a limiting factor for the efficiency of solar cells. Here, we show that strong coupling of organic molecules to a confined light mode can be used to strongly suppress photoisomerization, as well as other photochemical reactions, and thus convert molecules that normally show fast photodegradation into photostable forms. We find this to be especially efficient in the case of collective strong coupling, where the distribution of a single excitation over many molecules and the light mode leads to a collective protection effect that almost completely suppresses the photochemical reaction.
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Citations
Cites
Polariton-Mediated Energy Transfer between Organic Dyes in a Strongly Coupled Optical Microcavity
Coles, D. M., Somaschi, N., Michetti, P., Clark, C., Lagoudakis, P. G., Savvidis, P. G., & Lidzey, D. G. (2014) · Nature Materials · doi:10.1038/nmat3950 · Cited by 507
Douki, T., Reynaud-Angelin, A., Cadet, J., & Sage, E. (2003) · Biochemistry · doi:10.1021/bi034593c · Cited by 452
Cited by
Tilting a ground-state reactivity landscape by vibrational strong coupling
Thomas, A., Lethuillier-Karl, L., Nagarajan, K., Vergauwe, R. M. A., George, J., Chervy, T., Shalabney, A., Devaux, E., Genet, C., Moran, J., et al. (2019) · Science · doi:10.1126/science.aau7742 · Cited by 852
Novel Nanostructures and Materials for Strong Light–Matter Interactions
Baranov, D. G., Wersäll, M., Cuadra, J., Antosiewicz, T. J., & Shegai, T. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00674 · Cited by 531
Strong light–matter interactions: a new direction within chemistry
Hertzog, M., Wang, M., Mony, J., & Börjesson, K. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00193f · Cited by 444
Polaritonic Chemistry with Organic Molecules
Feist, J., Galego, J., & Garcia-Vidal, F. J. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00680 · Cited by 438
Self-citationTheoretical Advances in Polariton Chemistry and Molecular Cavity Quantum Electrodynamics
Mandal, A., Taylor, M. A. D., Weight, B. M., Koessler, E. R., Li, X., & Huo, P. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00855 · Cited by 270
Metadata
- Authors
- Galego, J., Garcia-Vidal, F. J., & Feist, J.
- Venue
- Nature Communications
- Published
- 2016-12-12
- Volume
- 7
- Issue
- 1
- Pages
- 13841-13841
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2433371754
- Cited by
- 343
- References
- 2
- FWCI
- 15.72
- Type
- journal article
- Language
- en
- Open access
- gold
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