The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Regulating the spatial distribution of metal nanoparticles within metal-organic frameworks to enhance catalytic efficiency
Open accessAbstract
Composites incorporating metal nanoparticles (MNPs) within metal-organic frameworks (MOFs) have broad applications in many fields. However, the controlled spatial distribution of the MNPs within MOFs remains a challenge for addressing key issues in catalysis, for example, the efficiency of catalysts due to the limitation of molecular diffusion within MOF channels. Here we report a facile strategy that enables MNPs to be encapsulated into MOFs with controllable spatial localization by using metal oxide both as support to load MNPs and as a sacrificial template to grow MOFs. This strategy is versatile to a variety of MNPs and MOF crystals. By localizing the encapsulated MNPs closer to the surface of MOFs, the resultant MNPs@MOF composites not only exhibit effective selectivity derived from MOF cavities, but also enhanced catalytic activity due to the spatial regulation of MNPs as close as possible to the MOF surface.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Horike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
Wu, H. B., Xia, B. Y., Yu, L., Yu, X.-Y., & Lou, X. W. (2015) · Nature Communications · doi:10.1038/ncomms7512 · Cited by 1,434
Cited by
Encapsulated Metal Nanoparticles for Catalysis
Gao, C., Lyu, F., & Yin, Y. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00237 · Cited by 855
Li, G., Zhao, S., Zhang, Y., & Tang, Z. (2018) · Advanced Materials · doi:10.1002/adma.201800702 · Cited by 521
Indra, A., Song, T., & Paik, U. (2018) · Advanced Materials · doi:10.1002/adma.201705146 · Cited by 507
Regulating the coordination structure of single-atom Fe-NxCy catalytic sites for benzene oxidation
Pan, Y., Chen, Y., Wu, K., Chen, Z., Liu, S., Cao, X., Cheong, W.-C., Meng, T., Luo, J., Zheng, L., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-12362-8 · Cited by 506
Multi‐shelled Hollow Metal–Organic Frameworks
Liu, W., Huang, J., Yang, Q., Wang, S., Sun, X., Zhang, W., Liu, J., & Huo, F. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201701604 · Cited by 367
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Metadata
- Authors
- Yang, Q., Liu, W., Wang, B., Zhang, W., Zeng, X., Zhang, C., Qin, Y., Sun, X., Wu, T., Liu, J., Huo, F., & Lu, J.
- Venue
- Nature Communications
- Published
- 2017-02-14
- Volume
- 8
- Issue
- 1
- Pages
- 14429-14429
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2588867799
- Cited by
- 241
- References
- 3
- FWCI
- 11.06
- Type
- journal article
- Language
- en
- Open access
- gold
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
