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A molecule-like PtAu24(SC6H13)18 nanocluster as an electrocatalyst for hydrogen production
Open accessAbstract
The theoretically predicted volcano plot for hydrogen production shows the best catalyst as the one that ensures that the hydrogen binding step is thermodynamically neutral. However, the experimental realization of this concept has suffered from the inherent surface heterogeneity of solid catalysts. It is even more challenging for molecular catalysts because of their complex chemical environment. Here, we report that the thermoneutral catalyst can be prepared by simple doping of a platinum atom into a molecule-like gold nanocluster. The catalytic activity of the resulting bimetallic nanocluster, PtAu 24(SC 6 H 13)18, for the hydrogen production is found to be significantly higher than reported catalysts. It is even better than the benchmarking platinum catalyst. The molecule-like bimetallic nanocluster represents a class of catalysts that bridge homogeneous and heterogeneous catalysis and may provide a platform for the discovery of finely optimized catalysts.
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Cites
Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
Recent advances in heterogeneous electrocatalysts for the hydrogen evolution reaction
Zeng, M., & Li, Y. (2015) · Journal of Materials Chemistry A · doi:10.1039/c5ta02974k · Cited by 1,294
Cited by
Liu, L., & Corma, A. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00733 · Cited by 689
Synthesis, Structure, Properties, and Applications of Bimetallic Nanoparticles of Noble Metals
Loza, K., Heggen, M., & Epple, M. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201909260 · Cited by 499
Wan, X., Wu, H. B., Guan, B. Y., Luan, D., & Lou, X. W. (. (2020) · Advanced Materials · doi:10.1002/adma.201901349 · Cited by 410
Pt‐Based Nanocrystal for Electrocatalytic Oxygen Reduction
Zhao, Z., Chen, C., Liu, Z., Huang, J., Wu, M., Liu, H., Li, Y., & Huang, Y. (2019) · Advanced Materials · doi:10.1002/adma.201808115 · Cited by 384
Tang, Q., Lee, Y., Li, D.-Y., Choi, W., Liu, C. W., Lee, D., & Jiang, D.-E. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b05591 · Cited by 382
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Metadata
- Authors
- Kwak, K., Choi, W., Tang, Q., Kim, M., Lee, Y., Jiang, D.-E., & Lee, D.
- Venue
- Nature Communications
- Published
- 2017-03-10
- Volume
- 8
- Issue
- 1
- Pages
- 14723-14723
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2593916779
- Cited by
- 372
- References
- 2
- FWCI
- 15.47
- Type
- journal article
- Language
- en
- Open access
- gold
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- Kwak, K., Choi, W., Tang, Q., Kim, M., Lee, Y., Jiang, D.-E., & Lee, D. (2017). A molecule-like PtAu24(SC6H13)18 nanocluster as an electrocatalyst for hydrogen production. Nature Communications. https://doi.org/10.1038/ncomms14723
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