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Polariton-mediated energy transfer between organic dyes in a strongly coupled optical microcavity
Abstract
Strongly coupled optical microcavities containing different exciton states permit the creation of hybrid-polariton modes that can be described in terms of a linear admixture of cavity-photon and the constituent excitons. Such hybrid states have been predicted to have optical properties that are different from their constituent parts, making them a test bed for the exploration of light-matter coupling. Here, we use strong coupling in an optical microcavity to mix the electronic transitions of two J-aggregated molecular dyes and use both non-resonant photoluminescence emission and photoluminescence excitation spectroscopy to show that hybrid-polariton states act as an efficient and ultrafast energy-transfer pathway between the two exciton states. We argue that this type of structure may act as a model system to study energy-transfer processes in biological light-harvesting complexes.
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“A smooth surface minimises light scattering and maintains the specular component of the reflection; in contrast, a rougher surface introduces significant diffuse scattering, diminishing the effective reflectance, especially when the roughness becomes comparable to a relevant fraction of the wavelength [242,243].”
From Metal Oxide Thin Films for Advanced Photonic Applications (2026) · cites this paper as [242]
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Metadata
- Authors
- Coles, D. M., Somaschi, N., Michetti, P., Clark, C., Lagoudakis, P. G., Savvidis, P. G., & Lidzey, D. G.
- Affiliations
- University of Sheffield (GB)
- Technische Universität Dresden (DE)
- Helia Photonics (United Kingdom) (GB)
- University of Southampton (GB)
- University of Crete (GR)
- Corresponding author
- Lidzey, David G.
- Venue
- Nature Materials
- Published
- 2014-05-04
- Volume
- 13
- Issue
- 7
- Pages
- 712-719
- ISSN
- 1476-1122 (ISSN-L)
- 1476-4660
- OpenAlex
- W2157928204
- Cited by
- 507
- References
- 49
- Citations by year
- 2026: 31 · 2025: 63 · 2024: 63 · 2023: 66 · 2022: 57 · 2021: 65 · 2020: 40 · 2019: 40 · 2018: 28 · 2017: 24 · 2016: 17 · 2015: 7 · 2014: 6
- FWCI
- 8.95
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Nature Materials (publishedVersion)
- PubMed (publishedVersion)
- ePrints Soton (University of Southampton) (acceptedVersion)
- Funders
- European Commission
- Engineering and Physical Sciences Research Council (EP/G063494/1, EP/G062404/1, EP/F026455/1)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Strong Light-Matter Interactions
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Photochemistry and Electron Transfer Studies
- Keywords
- exciton-polaritons, strong light-matter coupling, optical microcavities, energy transfer, organic dyes, Förster transfer, light-harvesting complexes, exciton mixing, ultrafast energy transfer
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