Cited by 484Zeolite Catalysis and SynthesisChemical Synthesis and CharacterizationMesoporous Materials and Catalysis

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Template-free nanosized faujasite-type zeolites

Awala, Hussein, Gilson, Jean-Pierre, Retoux, Richard, Boullay, Philippe, Goupil, Jean-Michel, Valtchev, Valentin, Mintova, Svetlana·2015·Nature Materials

DOI 10.1038/nmat4173

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Abstract

Nanosized faujasite (FAU) crystals have great potential as catalysts or adsorbents to more efficiently process present and forthcoming synthetic and renewable feedstocks in oil refining, petrochemistry and fine chemistry. Here, we report the rational design of template-free nanosized FAU zeolites with exceptional properties, including extremely small crystallites (10-15 nm) with a narrow particle size distribution, high crystalline yields (above 80%), micropore volumes (0.30 cm(3) g(-1)) comparable to their conventional counterparts (micrometre-sized crystals), Si/Al ratios adjustable between 1.1 and 2.1 (zeolites X or Y) and excellent thermal stability leading to superior catalytic performance in the dealkylation of a bulky molecule, 1,3,5-triisopropylbenzene, probing sites mostly located on the external surface of the nanosized crystals. Another important feature is their excellent colloidal stability, which facilitates a uniform dispersion on supports for applications in catalysis, sorption and thin-to-thick coatings.

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Authors: Awala, H., Gilson, J.-P., Retoux, R., Boullay, P., Goupil, J.-M., Valtchev, V., & Mintova, S.
Affiliations: Centre National de la Recherche Scientifique (FR)
Corresponding author: Mintova, Svetlana
ORCID: Awala, Hussein
Gilson, Jean-Pierre
Boullay, Philippe
Valtchev, Valentin
Mintova, Svetlana
Venue: Nature Materials
Publisher: Springer Science and Business Media LLC
Published: 2015-01-05
Volume: 14
Issue: 4
Pages: 447-451
ISSN: 1476-1122 (ISSN-L)
1476-4660
DOI: 10.1038/nmat4173
OpenAlex: W1994047443
Cited by: 484
References: 39
Citations by year: 2026: 20 · 2025: 41 · 2024: 51 · 2023: 42 · 2022: 40 · 2021: 45 · 2020: 56 · 2019: 40 · 2018: 50 · 2017: 42 · 2016: 38 · 2015: 19
FWCI: 20.40
Type: journal article
Language: en
Open access: closed
Licence: www.springer.com/tdm (tdm)
www.springer.com/tdm (vor)
Locations: Nature Materials (publishedVersion)
PubMed (publishedVersion)
HAL (submittedVersion)
Topics: Physical Sciences › Chemistry › Inorganic Chemistry › Zeolite Catalysis and Synthesis
Physical Sciences › Environmental Science › Waste Management and Disposal › Chemical Synthesis and Characterization
Physical Sciences › Materials Science › Materials Chemistry › Mesoporous Materials and Catalysis
Keywords: faujasite, nanosized zeolites, template-free synthesis, zeolite crystallization, Si/Al ratio, zeolite X, zeolite Y, thermal stability, dealkylation, 1,3,5-triisopropylbenzene, colloidal stability, particle size distribution, catalysts, adsorbents

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Template-free nanosized faujasite-type zeolites

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