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Sensing single remote nuclear spins
Open accessAbstract
The detection of single nuclear spins would be useful for fields ranging from basic science to quantum information technology. However, although sensing based on diamond defects and other methods have shown high sensitivity, they have not been capable of detecting single nuclear spins, and defect-based techniques further require strong defect-spin coupling. Here, we present the detection and identification of single and remote (13)C nuclear spins embedded in nuclear spin baths surrounding a single electron spin of a nitrogen-vacancy centre in diamond. We are able to amplify and detect the weak magnetic field noise (∼10 nT) from a single nuclear spin located ∼3 nm from the centre using dynamical decoupling control, and achieve a detectable hyperfine coupling strength as weak as ∼300 Hz. We also confirm the quantum nature of the coupling, and measure the spin-defect distance and the vector components of the nuclear field. The technique marks a step towards imaging, detecting and controlling nuclear spins in single molecules.
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Cites
Quantum register based on individual electronic and nuclear spin qubits in diamond
Dutt, M. V. G., Childress, L., Jiang, L., Togan, E., Maze, J., Jelezko, F., Zibrov, A. S., Hemmer, P. R., & Lukin, M. D. (2007) · Science · doi:10.1126/science.1139831 · Cited by 1,287
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Cited by
Coherent control of single spins in silicon carbide at room temperature
Widmann, M., Lee, S.-Y., Rendler, T., Son, N. T., Fedder, H., Paik, S., Yang, L.-P., Zhao, N., Yang, S., Booker, I., et al. (2015) · Nature Materials · doi:10.1038/nmat4145 · Cited by 668
Self-citationUnconditional quantum teleportation between distant solid-state quantum bits
Pfaff, W., Hensen, B. J., Bernien, H., van Dam, S. B., Blok, M. S., Taminiau, T. H., Tiggelman, M. J., Schouten, R. N., Markham, M., Twitchen, D. J., et al. (2014) · Science · doi:10.1126/science.1253512 · Cited by 528
Self-citationA ten-qubit solid-state spin register with quantum memory up to one minute
Bradley, C. E., Randall, J., Abobeih, M. H., Berrevoets, R. C., Degen, M. J., Bakker, M. A., Markham, M., Twitchen, D. J., & Taminiau, T. H. (2019) · Physical Review X · doi:10.1103/physrevx.9.031045 · Cited by 546
Self-citationOne-second coherence for a single electron spin coupled to a multi-qubit nuclear-spin environment
Abobeih, M. H., Cramer, J., Bakker, M. A., Kalb, N., Markham, M., Twitchen, D. J., & Taminiau, T. H. (2018) · Nature Communications · doi:10.1038/s41467-018-04916-z · Cited by 302
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Metadata
- Authors
- Zhao, N., Honert, J., Schmid, B., Klas, M., Isoya, J., Markham, M., Twitchen, D., Jelezko, F., Liu, R.-B., Fedder, H., & Wrachtrup, J.
- Venue
- Nature Nanotechnology
- Published
- 2012-09-02
- Volume
- 7
- Issue
- 10
- Pages
- 657-662
- ISSN
- 1748-3387 (ISSN-L)
- 1748-3395
- OpenAlex
- W2117142519
- Cited by
- 267
- References
- 1
- FWCI
- 13.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Zhao, N., Honert, J., Schmid, B., Klas, M., Isoya, J., Markham, M., Twitchen, D., Jelezko, F., Liu, R.-B., Fedder, H., & Wrachtrup, J. (2012). Sensing single remote nuclear spins. Nature Nanotechnology. https://doi.org/10.1038/nnano.2012.152
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