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Sub-cycle control of terahertz high-harmonic generation by dynamical Bloch oscillations

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Schubert, O., Hohenleutner, M., Langer, F., Urbanek, B., Lange, C., Huttner, U., Golde, D., Meier, T., Kira, M., Koch, S. W., Huber, R.·2014·Nature Photonics

Abstract

Ultrafast charge transport in strongly biased semiconductors is at the heart of high-speed electronics, electro-optics and fundamental solid-state physics1,2,3,4,5,6,7,8,9,10,11,12,13. Intense light pulses in the terahertz spectral range have opened fascinating vistas14,15,16,17,18,19,20,21. Because terahertz photon energies are far below typical electronic interband resonances, a stable electromagnetic waveform may serve as a precisely adjustable bias5,11,17,19. Novel quantum phenomena have been anticipated for terahertz amplitudes, reaching atomic field strengths8,9,10. We exploit controlled (multi-)terahertz waveforms with peak fields of 72 MV cm−1 to drive coherent interband polarization combined with dynamical Bloch oscillations in semiconducting gallium selenide. These dynamics entail the emission of phase-stable high-harmonic transients, covering the entire terahertz-to-visible spectral domain between 0.1 and 675 THz. Quantum interference of different ionization paths of accelerated charge carriers is controlled via the waveform of the driving field and explained by a quantum theory of inter- and intraband dynamics. Our results pave the way towards all-coherent terahertz-rate electronics. Terahertz waveforms with peak fields of 72 MV cm−1 and a central frequency of 30 THz drive interband polarization in bulk GaSe off-resonantly and accelerate excited electron–hole pairs, inducing dynamical Bloch oscillations. This results in the emission of phase-stable, high-harmonic transients over the whole frequency range of 0.1–675 THz.

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Metadata

Authors
Schubert, O., Hohenleutner, M., Langer, F., Urbanek, B., Lange, C., Huttner, U., Golde, D., Meier, T., Kira, M., Koch, S. W., & Huber, R.
Venue
Nature Photonics
Published
2014-01-19
Volume
8
Issue
2
Pages
119-123
ISSN
  • 1749-4885 (ISSN-L)
  • 1749-4893
OpenAlex
W2040677847
Cited by
1,026
References
5
FWCI
36.60
Type
journal article
Language
en
Open access
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CoChat. (2026). Citation check: Sub-cycle control of terahertz high-harmonic generation by dynamical Bloch oscillations. https://app.cochat.ai/papers/10.1038/nphoton.2013.349
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Schubert, O., Hohenleutner, M., Langer, F., Urbanek, B., Lange, C., Huttner, U., Golde, D., Meier, T., Kira, M., Koch, S. W., & Huber, R. (2014). Sub-cycle control of terahertz high-harmonic generation by dynamical Bloch oscillations. Nature Photonics. https://doi.org/10.1038/nphoton.2013.349

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