The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Organosulfide-plasticized solid-electrolyte interphase layer enables stable lithium metal anodes for long-cycle lithium-sulfur batteries
Open accessAbstract
Lithium metal is a promising anode candidate for the next-generation rechargeable battery due to its highest specific capacity (3860 mA h g−1) and lowest potential, but low Coulombic efficiency and formation of lithium dendrites hinder its practical application. Here, we report a self-formed flexible hybrid solid-electrolyte interphase layer through co-deposition of organosulfides/organopolysulfides and inorganic lithium salts using sulfur-containing polymers as an additive in the electrolyte. The organosulfides/organopolysulfides serve as “plasticizer” in the solid-electrolyte interphase layer to improve its mechanical flexibility and toughness. The as-formed robust solid-electrolyte interphase layers enable dendrite-free lithium deposition and significantly improve Coulombic efficiency (99% over 400 cycles at a current density of 2 mA cm−2). A lithium-sulfur battery based on this strategy exhibits long cycling life (1000 cycles) and good capacity retention. This study reveals an avenue to effectively fabricate stable solid-electrolyte interphase layer for solving the issues associated with lithium metal anodes.
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Cites
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Li, G., Liu, Z., Huang, Q., Gao, Y., Regula, M., Wang, D., Chen, L.-Q., & Wang, D. (2018) · Nature Energy · doi:10.1038/s41560-018-0276-z · Cited by 444
Self-citationLithium anode stable in air for low-cost fabrication of a dendrite-free lithium battery
Shen, X., Li, Y., Qian, T., Liu, J., Zhou, J., Yan, C., & Goodenough, J. B. (2019) · Nature Communications · doi:10.1038/s41467-019-08767-0 · Cited by 386
Designable ultra-smooth ultra-thin solid-electrolyte interphases of three alkali metal anodes
Gu, Y., Wang, W.-W., Li, Y.-J., Wu, Q.-H., Tang, S., Yan, J.-W., Zheng, M.-S., Wu, D.-Y., Fan, C.-H., Hu, W.-Q., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-03466-8 · Cited by 355
Zhang, X., Li, T., Li, B., Zhang, R., Shi, P., Yan, C., Huang, J., & Zhang, Q. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201911724 · Cited by 313
New Insight on the Role of Electrolyte Additives in Rechargeable Lithium Ion Batteries
Ming, J., Cao, Z., Wu, Y., Wahyudi, W., Wang, W., Guo, X., Cavallo, L., Hwang, J.-Y., Shamim, A., Li, L.-J., et al. (2019) · ACS Energy Letters · doi:10.1021/acsenergylett.9b01441 · Cited by 294
Metadata
- Authors
- Li, G., Gao, Y., He, X., Huang, Q., Chen, S., Kim, S. H., & Wang, D.
- Venue
- Nature Communications
- Published
- 2017-10-11
- Volume
- 8
- Issue
- 1
- Pages
- 850-850
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2763629673
- Cited by
- 314
- References
- 1
- FWCI
- 15.66
- Type
- journal article
- Language
- en
- Open access
- gold
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- Li, G., Gao, Y., He, X., Huang, Q., Chen, S., Kim, S. H., & Wang, D. (2017). Organosulfide-plasticized solid-electrolyte interphase layer enables stable lithium metal anodes for long-cycle lithium-sulfur batteries. Nature Communications. https://doi.org/10.1038/s41467-017-00974-x
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