The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Two-dimensional metallic tantalum disulfide as a hydrogen evolution catalyst
Open accessAbstract
Two-dimensional metallic transition metal dichalcogenides are emerging as prototypes for uncovering fundamental physical phenomena, such as superconductivity and charge-density waves, as well as for engineering-related applications. However, the batch production of such envisioned transition metal dichalcogenides remains challenging, which has hindered the aforementioned explorations. Herein, we fabricate thickness-tunable tantalum disulfide flakes and centimetre-sized ultrathin films on an electrode material of gold foil via a facile chemical vapour deposition route. Through temperature-dependent Raman characterization, we observe the transition from nearly commensurate to commensurate charge-density wave phases with our ultrathin tantalum disulfide flakes. We have obtained high hydrogen evolution reaction efficiency with the as-grown tantalum disulfide flakes directly synthesized on gold foils comparable to traditional platinum catalysts. This work could promote further efforts for exploring new efficient catalysts in the large materials family of metallic transition metal dichalcogenides, as well as exploiting their applications towards more versatile applications.
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Citations
Cites
Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts
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Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
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Layer-Dependent Electrocatalysis of MoS2 for Hydrogen Evolution
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Self-citationShi, J., Ma, D., Han, G.-F., Zhang, Y., Ji, Q., Gao, T., Sun, J., Song, X., Li, C., Zhang, Y., et al. (2014) · ACS Nano · doi:10.1021/nn503211t · Cited by 459
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Cited by
Chandrasekaran, S., Yao, L., Deng, L., Bowen, C., Zhang, Y., Chen, S., Lin, Z., Peng, F., & Zhang, P. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00664d · Cited by 1,199
Self-citationRecent Advances in Design of Electrocatalysts for High‐Current‐Density Water Splitting
Luo, Y., Zhang, Z., Chhowalla, M., & Liu, B. (2022) · Advanced Materials · doi:10.1002/adma.202108133 · Cited by 854
Self-citationPreparation of 2D material dispersions and their applications
Cai, X., Luo, Y., Liu, B., & Cheng, H.-M. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00254a · Cited by 665
Wang, M., Zhang, L., He, Y., & Zhu, H. (2021) · Journal of Materials Chemistry A · doi:10.1039/d0ta12152e · Cited by 648
Ultrahigh-current-density niobium disulfide catalysts for hydrogen evolution
Yang, J., Mohmad, A. R., Wang, Y., Fullon, R., Song, X., Zhao, F., Bozkurt, I., Augustin, M., Santos, E. J. G., Shin, H. S., et al. (2019) · Nature Materials · doi:10.1038/s41563-019-0463-8 · Cited by 401
Metadata
- Authors
- Shi, J., Wang, X., Zhang, S., Xiao, L., Huan, Y., Gong, Y., Zhang, Z., Li, Y., Zhou, X., Hong, M., Fang, Q., Zhang, Q., Liu, X., Gu, L., Liu, Z., & Zhang, Y.
- Venue
- Nature Communications
- Published
- 2017-10-16
- Volume
- 8
- Issue
- 1
- Pages
- 958-958
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2762125931
- Cited by
- 239
- References
- 7
- FWCI
- 10.84
- Type
- journal article
- Language
- en
- Open access
- gold
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- Shi, J., Wang, X., Zhang, S., Xiao, L., Huan, Y., Gong, Y., Zhang, Z., Li, Y., Zhou, X., Hong, M., Fang, Q., Zhang, Q., Liu, X., Gu, L., Liu, Z., & Zhang, Y. (2017). Two-dimensional metallic tantalum disulfide as a hydrogen evolution catalyst. Nature Communications. https://doi.org/10.1038/s41467-017-01089-z
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