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A two-dimensional Fe-doped SnS2 magnetic semiconductor

Open access
Li, Bo, Xing, Tao, Zhong, Mianzeng, Huang, Le, Lei, Na, Zhang, Jun, Li, Jingbo, Wei, Zhongming·2017·Nature Communications

Abstract

Magnetic two-dimensional materials have attracted considerable attention for their significant potential application in spintronics. In this study, we present a high-quality Fe-doped SnS 2 monolayer exfoliated using a micromechanical cleavage method. Fe atoms were doped at the Sn atom sites, and the Fe contents are ∼2.1%, 1.5%, and 1.1%. The field-effect transistors based on the Fe 0.021 Sn 0.979 S 2 monolayer show n-type behavior and exhibit high optoelectronic performance. Magnetic measurements show that pure SnS 2 is diamagnetic, whereas Fe 0.021 Sn 0.979 S 2 exhibits ferromagnetic behavior with a perpendicular anisotropy at 2 K and a Curie temperature of ~31 K. Density functional theory calculations show that long-range ferromagnetic ordering in the Fe-doped SnS 2 monolayer is energetically stable, and the estimated Curie temperature agrees well with the results of our experiment. The results suggest that Fe-doped SnS 2 has significant potential in future nanoelectronic, magnetic, and optoelectronic applications.

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Metadata

Authors
Li, B., Xing, T., Zhong, M., Huang, L., Lei, N., Zhang, J., Li, J., & Wei, Z.
Venue
Nature Communications
Published
2017-12-05
Volume
8
Issue
1
Pages
1958-1958
ISSN
2041-1723 (ISSN-L)
OpenAlex
W2768331633
Cited by
423
References
36
FWCI
17.05
Type
journal article
Language
en
Open access
gold

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CoChat. (2026). Citation check: A two-dimensional Fe-doped SnS2 magnetic semiconductor. https://app.cochat.ai/papers/10.1038/s41467-017-02077-z
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Li, B., Xing, T., Zhong, M., Huang, L., Lei, N., Zhang, J., Li, J., & Wei, Z. (2017). A two-dimensional Fe-doped SnS2 magnetic semiconductor. Nature Communications. https://doi.org/10.1038/s41467-017-02077-z

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