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Manipulation of facet orientation in hybrid perovskite polycrystalline films by cation cascade
Open accessAbstract
Crystal orientations in multiple orders correlate to the properties of polycrystalline materials, and it is critical to manipulate these microstructural arrangements to enhance device performance. Herein, we report a controllable approach to manipulate the facet orientation within the ABX 3 hybrid perovskites polycrystalline films by cation cascade doping at A-site. Two-dimensional synchrotron radiation grazing incidence wide-angle X-ray scattering is employed to probe the crystal orientations in multiple orders in mixed perovskites thin films, revealing a general pattern to guide crystal planes stacking upon extrinsic doping during crystallization. Different from previous studies, this method enables to adjust the crystal stacking mode of certain crystallographic planes in polycrystalline perovskites. Moreover, the preferred facet orientation is found to facilitate photocarrier transport across the absorber and pertaining interface in the resultant PV device, which provides an exemplary paradigm for further explorations that relate to the microstructures of hybrid perovskite materials and relevant optoelectronics.
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Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Impact of microstructure on local carrier lifetime in perovskite solar cells
de Quilettes, D. W., Vorpahl, S. M., Stranks, S. D., Nagaoka, H., Eperon, G. E., Ziffer, M. E., Snaith, H. J., & Ginger, D. S. (2015) · Science · doi:10.1126/science.aaa5333 · Cited by 2,198
Cited by
Crystal Facet Engineering of Photoelectrodes for Photoelectrochemical Water Splitting
Wang, S., Liu, G., & Wang, L. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00584 · Cited by 847
Interfacial Residual Stress Relaxation in Perovskite Solar Cells with Improved Stability
Wang, H., Zhu, C., Liu, L., Ma, S., Liu, P., Wu, J., Shi, C., Du, Q., Hao, Y., Xiang, S., et al. (2019) · Advanced Materials · doi:10.1002/adma.201904408 · Cited by 499
Self-citationA general approach to high-efficiency perovskite solar cells by any antisolvent
Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y. (2021) · Nature Communications · doi:10.1038/s41467-021-22049-8 · Cited by 451
Toward Understanding Space-Charge Limited Current Measurements on Metal Halide Perovskites
Duijnstee, E. A., Ball, J. M., Le Corre, V. M., Koster, L. J. A., Snaith, H. J., & Lim, J. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.9b02720 · Cited by 437
Photovoltaically top-performing perovskite crystal facets
Ma, C., Kang, M.-C., Lee, S.-H., Kwon, S. J., Cha, H.-W., Yang, C.-W., & Park, N.-G. (2022) · Joule · doi:10.1016/j.joule.2022.09.012 · Cited by 349
Metadata
- Authors
- Zheng, G., Zhu, C., Ma, J., Zhang, X., Tang, G., Li, R., Chen, Y., Li, L., Hu, J., Hong, J., Chen, Q., Gao, X., & Zhou, H.
- Venue
- Nature Communications
- Published
- 2018-07-18
- Volume
- 9
- Issue
- 1
- Pages
- 2793-2793
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2870524276
- Cited by
- 278
- References
- 2
- FWCI
- 10.63
- Type
- journal article
- Language
- en
- Open access
- gold
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