The DOI matches its Crossref record; 54 of the 54 references it cites were found in a registry or an index.
A general approach to high-efficiency perovskite solar cells by any antisolvent
Open accessAbstract
Deposition of perovskite films by antisolvent engineering is a highly common method employed in perovskite photovoltaics research. Herein, we report on a general method that allows for the fabrication of highly efficient perovskite solar cells by any antisolvent via manipulation of the antisolvent application rate. Through detailed structural, compositional, and microstructural characterization of perovskite layers fabricated by 14 different antisolvents, we identify two key factors that influence the quality of the perovskite layer: the solubility of the organic precursors in the antisolvent and its miscibility with the host solvent(s) of the perovskite precursor solution, which combine to produce rate-dependent behavior during the antisolvent application step. Leveraging this, we produce devices with power conversion efficiencies (PCEs) that exceed 21% using a wide range of antisolvents. Moreover, we demonstrate that employing the optimal antisolvent application procedure allows for highly efficient solar cells to be fabricated from a broad range of precursor stoichiometries.
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Cites
Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites
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Structural absorption by barbule microstructures of super black bird of paradise feathers
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Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
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National Renewable Energy Laboratory
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Self-citationEfficient luminescent solar cells based on tailored mixed-cation perovskites
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Metadata
- Authors
- Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y.
- Venue
- Nature Communications
- Published
- 2021-03-25
- Volume
- 12
- Issue
- 1
- Pages
- 1878-1878
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3129036993
- Cited by
- 451
- References
- 54
- FWCI
- 21.75
- Type
- journal article
- Language
- en
- Open access
- gold
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- Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y. (2021). A general approach to high-efficiency perovskite solar cells by any antisolvent. Nature Communications. https://doi.org/10.1038/s41467-021-22049-8
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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