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The DOI matches its Crossref record; 54 of the 54 references it cites were found in a registry or an index.

A general approach to high-efficiency perovskite solar cells by any antisolvent

Open access
Taylor, Alexander D., Sun, Qing, Goetz, Katelyn P., An, Qingzhi, Schramm, Tim, Hofstetter, Yvonne, Litterst, Maximillian, Paulus, Fabian, Vaynzof, Yana·2021·Nature Communications

Abstract

Deposition of perovskite films by antisolvent engineering is a highly common method employed in perovskite photovoltaics research. Herein, we report on a general method that allows for the fabrication of highly efficient perovskite solar cells by any antisolvent via manipulation of the antisolvent application rate. Through detailed structural, compositional, and microstructural characterization of perovskite layers fabricated by 14 different antisolvents, we identify two key factors that influence the quality of the perovskite layer: the solubility of the organic precursors in the antisolvent and its miscibility with the host solvent(s) of the perovskite precursor solution, which combine to produce rate-dependent behavior during the antisolvent application step. Leveraging this, we produce devices with power conversion efficiencies (PCEs) that exceed 21% using a wide range of antisolvents. Moreover, we demonstrate that employing the optimal antisolvent application procedure allows for highly efficient solar cells to be fabricated from a broad range of precursor stoichiometries.

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Metadata

Authors
Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y.
Venue
Nature Communications
Published
2021-03-25
Volume
12
Issue
1
Pages
1878-1878
ISSN
2041-1723 (ISSN-L)
OpenAlex
W3129036993
Cited by
451
References
54
FWCI
21.75
Type
journal article
Language
en
Open access
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CoChat. (2026). Citation check: A general approach to high-efficiency perovskite solar cells by any antisolvent. https://app.cochat.ai/papers/10.1038/s41467-021-22049-8
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Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y. (2021). A general approach to high-efficiency perovskite solar cells by any antisolvent. Nature Communications. https://doi.org/10.1038/s41467-021-22049-8

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