The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Selective conversion of CO2 and H2 into aromatics
Open accessAbstract
Transformation of greenhouse gas CO 2 and renewable H 2 into fuels and commodity chemicals is recognized as a promising route to store fluctuating renewable energy. Although several C 1 chemicals, olefins, and gasoline have been successfully synthesized by CO 2 hydrogenation, selective conversion of CO 2 and H 2 into aromatics is still challenging due to the high unsaturation degree and complex structures of aromatics. Here we report a composite catalyst of ZnAlOx and H-ZSM-5 which yields high aromatics selectivity (73.9%) with extremely low CH 4 selectivity (0.4%) among the carbon products without CO. Methanol and dimethyl ether, which are synthesized by hydrogenation of formate species formed on ZnAlOx surface, are transmitted to H-ZSM-5 and subsequently converted into olefins and finally aromatics. Furthermore, 58.1% p-xylene in xylenes is achieved over the composite catalyst containing Si-H-ZSM-5. ZnAlOx&H-ZSM-5 suggests a promising application in manufacturing aromatics from CO 2 and H 2.
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Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
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Vogt, C., Monai, M., Kramer, G. J., & Weckhuysen, B. M. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0244-4 · Cited by 636
Pan, X., Jiao, F., Miao, D., & Bao, X. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01012 · Cited by 423
Significant Advances in C1 Catalysis: Highly Efficient Catalysts and Catalytic Reactions
Bao, J., Yang, G., Yoneyama, Y., & Tsubaki, N. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b03924 · Cited by 367
Highly Active ZnO-ZrO2 Aerogels Integrated with H-ZSM-5 for Aromatics Synthesis from Carbon Dioxide
Zhou, C., Shi, J., Zhou, W., Cheng, K., Zhang, Q., Kang, J., & Wang, Y. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b04309 · Cited by 361
Metadata
- Authors
- Ni, Y., Chen, Z., Fu, Y., Liu, Y., Zhu, W., & Liu, Z.
- Venue
- Nature Communications
- Published
- 2018-08-27
- Volume
- 9
- Issue
- 1
- Pages
- 3457-3457
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2888756095
- Cited by
- 484
- References
- 1
- FWCI
- 8.47
- Type
- journal article
- Language
- en
- Open access
- gold
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