The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Solubility-mediated sustained release enabling nitrate additive in carbonate electrolytes for stable lithium metal anode
Open accessAbstract
The physiochemical properties of the solid-electrolyte interphase, primarily governed by electrolyte composition, have a profound impact on the electrochemical cycling of metallic lithium. Herein, we discover that the effect of nitrate anions on regulating lithium deposition previously known in ether-based electrolytes can be extended to carbonate-based systems, which dramatically alters the nuclei from dendritic to spherical, albeit extremely limited solubility. This is attributed to the preferential reduction of nitrate during solid-electrolyte interphase formation, and the mechanisms behind which are investigated based on the structure, ion-transport properties, and charge transfer kinetics of the modified interfacial environment. To overcome the solubility barrier, a solubility-mediated sustained-release methodology is introduced, in which nitrate nanoparticles are encapsulated in porous polymer gel and can be steadily dissolved during battery operation to maintain a high concentration at the electroplating front. As such, effective dendrite suppression and remarkably enhanced cycling stability are achieved in corrosive carbonate electrolytes.
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Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Atomic structure of sensitive battery materials and interfaces revealed by cryo–electron microscopy
Li, Y., Li, Y., Pei, A., Yan, K., Sun, Y., Wu, C.-L., Joubert, L.-M., Chin, R., Koh, A. L., Yu, Y., et al. (2017) · Science · doi:10.1126/science.aam6014 · Cited by 1,547
Self-citationWang, X., Zhang, M., Alvarado, J., Wang, S., Sina, M., Lu, B., Bouwer, J., Xu, W., Xiao, J., Zhang, J.-G., et al. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b03606 · Cited by 409
Cited by
Alleviation of Dendrite Formation on Zinc Anodes via Electrolyte Additives
Guo, X., Zhang, Z., Li, J., Luo, N., Chai, G.-L., Miller, T. S., Lai, F., Shearing, P., Brett, D. J. L., Han, D., et al. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02371 · Cited by 594
Lithium Metal Batteries Enabled by Synergetic Additives in Commercial Carbonate Electrolytes
Piao, N., Liu, S., Zhang, B., Ji, X., Fan, X., Wang, L., Wang, P.-F., Jin, T., Liou, S.-C., Yang, H., et al. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.1c00365 · Cited by 355
Xia, Y., Zhou, P., Kong, X., Tian, J., Zhang, W., Yan, S., Hou, W.-H., Zhou, H.-Y., Dong, H., Chen, X., et al. (2023) · Nature Energy · doi:10.1038/s41560-023-01282-z · Cited by 346
Corrosion of lithium metal anodes during calendar ageing and its microscopic origins
Boyle, D. T., Huang, W., Wang, H., Li, Y., Chen, H., Yu, Z., Zhang, W., Bao, Z., & Cui, Y. (2021) · Nature Energy · doi:10.1038/s41560-021-00787-9 · Cited by 334
Self-citationZhang, X., Li, T., Li, B., Zhang, R., Shi, P., Yan, C., Huang, J., & Zhang, Q. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201911724 · Cited by 313
Metadata
- Authors
- Liu, Y., Lin, D., Li, Y., Chen, G., Pei, A., Nix, O., Li, Y., & Cui, Y.
- Venue
- Nature Communications
- Published
- 2018-09-07
- Volume
- 9
- Issue
- 1
- Pages
- 3656-3656
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2891628382
- Cited by
- 570
- References
- 4
- FWCI
- 19.95
- Type
- journal article
- Language
- en
- Open access
- gold
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- Liu, Y., Lin, D., Li, Y., Chen, G., Pei, A., Nix, O., Li, Y., & Cui, Y. (2018). Solubility-mediated sustained release enabling nitrate additive in carbonate electrolytes for stable lithium metal anode. Nature Communications. https://doi.org/10.1038/s41467-018-06077-5
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