The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Non defect-stabilized thermally stable single-atom catalyst
Open accessAbstract
Surface-supported isolated atoms in single-atom catalysts (SACs) are usually stabilized by diverse defects. The fabrication of high-metal-loading and thermally stable SACs remains a formidable challenge due to the difficulty of creating high densities of underpinning stable defects. Here we report that isolated Pt atoms can be stabilized through a strong covalent metal-support interaction (CMSI) that is not associated with support defects, yielding a high-loading and thermally stable SAC by trapping either the already deposited Pt atoms or the PtO 2 units vaporized from nanoparticles during high-temperature calcination. Experimental and computational modeling studies reveal that iron oxide reducibility is crucial to anchor isolated Pt atoms. The resulting high concentrations of single atoms enable specific activities far exceeding those of conventional nanoparticle catalysts. This non defect-stabilization strategy can be extended to non-reducible supports by simply doping with iron oxide, thus paving a new way for constructing high-loading SACs for diverse industrially important catalytic reactions.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
Kresse, G., & Furthmüller, J. (1996) · Physical Review B · doi:10.1103/physrevb.54.11169 · Cited by 123,652
From ultrasoft pseudopotentials to the projector augmented-wave method
Kresse, G., & Joubert, D. (1999) · Physical Review B · doi:10.1103/physrevb.59.1758 · Cited by 85,307
Fei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Self-citation
Cited by
Iridium Single Atoms Coupling with Oxygen Vacancies Boosts Oxygen Evolution Reaction in Acid Media
Yin, J., Jin, J., Lu, M., Huang, B., Zhang, H., Peng, Y., Xi, P., & Yan, C.-H. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c05050 · Cited by 545
Stable and Efficient Single-Atom Zn Catalyst for CO2 Reduction to CH4
Han, L., Song, S., Liu, M., Yao, S., Liang, Z., Cheng, H., Ren, Z., Liu, W., Lin, R., Qi, G., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b12111 · Cited by 538
Self-citationRecent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Self-citationZhuang, Z., Li, Y., Yu, R., Xia, L., Yang, J., Lang, Z., Zhu, J., Huang, J., Wang, J., Wang, Y., et al. (2022) · Nature Catalysis · doi:10.1038/s41929-022-00764-9 · Cited by 325
Hejazi, S., Mohajernia, S., Osuagwu, B., Zoppellaro, G., Andryskova, P., Tomanec, O., Kment, S., Zbořil, R., & Schmuki, P. (2020) · Advanced Materials · doi:10.1002/adma.201908505 · Cited by 319
Metadata
- Authors
- Lang, R., Xi, W., Liu, J.-C., Cui, Y.-T., Li, T., Lee, A. F., Chen, F., Chen, Y., Li, L., Li, L., Lin, J., Miao, S., Liu, X., Wang, A.-Q., Wang, X., Luo, J., Qiao, B., Li, J., & Zhang, T.
- Venue
- Nature Communications
- Published
- 2019-01-16
- Volume
- 10
- Issue
- 1
- Pages
- 234-234
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2911133971
- Cited by
- 642
- References
- 5
- FWCI
- 30.39
- Type
- journal article
- Language
- en
- Open access
- gold
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
How to cite
Cite CoChat for the checks on this page, and the paper for its own findings.
- This page
- CoChat. (2026). Citation check: Non defect-stabilized thermally stable single-atom catalyst. https://app.cochat.ai/papers/10.1038/s41467-018-08136-3
- The paper
- Lang, R., Xi, W., Liu, J.-C., Cui, Y.-T., Li, T., Lee, A. F., Chen, F., Chen, Y., Li, L., Li, L., Lin, J., Miao, S., Liu, X., Wang, A.-Q., Wang, X., Luo, J., Qiao, B., Li, J., & Zhang, T. (2019). Non defect-stabilized thermally stable single-atom catalyst. Nature Communications. https://doi.org/10.1038/s41467-018-08136-3
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
