The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
Stable radical anions generated from a porous perylenediimide metal-organic framework for boosting near-infrared photothermal conversion
Open accessAbstract
Radical anions of electron-deficient systems are widely used, but are easily reoxidized upon exposure to air. Therefore, the stabilization of radical anions under ambient conditions is of great significance, but still remains a scientific challenge. Herein, perylenediimide is employed to prepare a crystalline metal-organic framework for stabilizing radical anions without extensive chemical modification. The porous, three-dimensional framework of perylenediimide can trap electron donors such as amine vapors and produce radical anions in-situ through photo-induced electron transfer. The radical anions are protected against quenching by shielding effect in air and remain unobstructed in air for at least a month. Because of the high yield and stability of the radical anions, which are the basis for near-infrared photothermal conversion, the framework shows high near-infrared photothermal conversion efficiency (η = 52.3%). The work provides an efficient and simple method towards ambient stable radical anions and affords a promising material for photothermal therapy.
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Metadata
- Authors
- Lü, B., Chen, Y., Li, P., Wang, B., Müllen, K., & Yin, M.
- Venue
- Nature Communications
- Published
- 2019-02-15
- Volume
- 10
- Issue
- 1
- Pages
- 767-767
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2914513207
- Cited by
- 454
- References
- 37
- FWCI
- 17.11
- Type
- journal article
- Language
- en
- Open access
- gold
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- Lü, B., Chen, Y., Li, P., Wang, B., Müllen, K., & Yin, M. (2019). Stable radical anions generated from a porous perylenediimide metal-organic framework for boosting near-infrared photothermal conversion. Nature Communications. https://doi.org/10.1038/s41467-019-08434-4
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