The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Room temperature CO2 reduction to solid carbon species on liquid metals featuring atomically thin ceria interfaces
Open accessAbstract
Negative carbon emission technologies are critical for ensuring a future stable climate. However, the gaseous state of CO 2 does render the indefinite storage of this greenhouse gas challenging. Herein, we created a liquid metal electrocatalyst that contains metallic elemental cerium nanoparticles, which facilitates the electrochemical reduction of CO 2 to layered solid carbonaceous species, at a low onset potential of −310 mV vs CO 2/C. We exploited the formation of a cerium oxide catalyst at the liquid metal/electrolyte interface, which together with cerium nanoparticles, promoted the room temperature reduction of CO 2. Due to the inhibition of van der Waals adhesion at the liquid interface, the electrode was remarkably resistant to deactivation via coking caused by solid carbonaceous species. The as-produced solid carbonaceous materials could be utilised for the fabrication of high-performance capacitor electrodes. Overall, this liquid metal enabled electrocatalytic process at room temperature may result in a viable negative emission technology.
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Cites
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Research Opportunities for CO2 Utilization and Negative Emissions at the Gigatonne Scale
Majumdar, A., & Deutch, J. (2018) · Joule · doi:10.1016/j.joule.2018.04.018 · Cited by 89
Cited by
Attributes, Fabrication, and Applications of Gallium‐Based Liquid Metal Particles
Lin, Y., Genzer, J., & Dickey, M. D. (2020) · Advanced Science · doi:10.1002/advs.202000192 · Cited by 503
Self-citationLiquid metal for high-entropy alloy nanoparticles synthesis
Cao, G., Liang, J., Guo, Z., Yang, K., Wang, G., Wang, H., Wan, X., Li, Z., Bai, Y., Zhang, Y., et al. (2023) · Nature · doi:10.1038/s41586-023-06082-9 · Cited by 375
Wang, Y., Liu, Y., Liu, W., Wu, J., Li, Q., Feng, Q., Chen, Z., Xiong, X., Wang, D., & Lei, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02833a · Cited by 303
Liquid Metal‐Based Soft Electronics for Wearable Healthcare
Park, Y., Lee, G., Jang, J., Yun, S. M., Kim, E., & Park, J. (2021) · Advanced Healthcare Materials · doi:10.1002/adhm.202002280 · Cited by 258
Metadata
- Authors
- Esrafilzadeh, D., Zavabeti, A., Jalili, R., Atkin, P., Choi, J., Carey, B. J., Brkljača, R., O’Mullane, A. P., Dickey, M. D., Officer, D. L., MacFarlane, D. R., Daeneke, T., & Kalantar-Zadeh, K.
- Venue
- Nature Communications
- Published
- 2019-02-26
- Volume
- 10
- Issue
- 1
- Pages
- 865-865
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2917284153
- Cited by
- 279
- References
- 3
- FWCI
- 6.91
- Type
- journal article
- Language
- en
- Open access
- gold
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- Esrafilzadeh, D., Zavabeti, A., Jalili, R., Atkin, P., Choi, J., Carey, B. J., Brkljača, R., O’Mullane, A. P., Dickey, M. D., Officer, D. L., MacFarlane, D. R., Daeneke, T., & Kalantar-Zadeh, K. (2019). Room temperature CO2 reduction to solid carbon species on liquid metals featuring atomically thin ceria interfaces. Nature Communications. https://doi.org/10.1038/s41467-019-08824-8
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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