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Cross-linked beta alumina nanowires with compact gel polymer electrolyte coating for ultra-stable sodium metal battery
Open accessAbstract
Sodium metal batteries have potentially high energy densities, but severe sodium-dendrite growth and side reactions prevent their practical applications, especially at high temperatures. Herein, we design an inorganic ionic conductor/gel polymer electrolyte composite, where uniformly cross-linked beta alumina nanowires are compactly coated by a poly(vinylidene fluoride-co-hexafluoropropylene)-based gel polymer electrolyte through their strong molecular interactions. These beta alumina nanowires combined with the gel polymer layer create dense and homogeneous solid-liquid hybrid sodium-ion transportation channels through and along the nanowires, which promote uniform sodium deposition and formation of a stable and flat solid electrolyte interface on the sodium metal anode. Side reactions between the sodium metal and liquid electrolyte, as well as sodium dendrite formation, are successfully suppressed, especially at 60 °C. The sodium vanadium phosphate/sodium full cells with composite electrolyte exhibit 95.3% and 78.8% capacity retention after 1000 cycles at 1 C at 25 °C and 60 °C, respectively.
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Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Cited by
Liu, W., Liu, P., & Mitlin, D. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202002297 · Cited by 687
Shi, P., Ma, J., Liu, M., Guo, S., Huang, Y., Wang, S., Zhang, L., Chen, L., Yang, K., Liu, X., et al. (2023) · Nature Nanotechnology · doi:10.1038/s41565-023-01341-2 · Cited by 578
Self-citationGel polymer electrolytes for rechargeable batteries toward wide-temperature applications
Zhou, X., Zhou, Y., Yu, L., Qi, L., Oh, K.-S., Hu, P., Lee, S.-Y., & Chen, C. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00551h · Cited by 333
Huang, J., Wu, K., Xu, G., Wu, M., Dou, S., & Wu, C. (2023) · Chemical Society Reviews · doi:10.1039/d2cs01029a · Cited by 304
Su, Y., Rong, X., Gao, A., Liu, Y., Li, J., Mao, M., Qi, X., Chai, G., Zhang, Q., Suo, L., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-31792-5 · Cited by 293
Metadata
- Authors
- Lei, D., He, Y.-B., Huang, H., Yuan, Y., Zhong, G., Zhao, Q., Hao, X., Zhang, D., Lai, C., Zhang, S., Ma, J., Wei, Y., Yu, Q., Lv, W., Yu, Y., Li, B., Yang, Q.-H., Yang, Y., Lu, J., & Kang, F.
- Venue
- Nature Communications
- Published
- 2019-09-18
- Volume
- 10
- Issue
- 1
- Pages
- 4244-4244
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2974608400
- Cited by
- 332
- References
- 1
- FWCI
- 14.54
- Type
- journal article
- Language
- en
- Open access
- gold
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- Lei, D., He, Y.-B., Huang, H., Yuan, Y., Zhong, G., Zhao, Q., Hao, X., Zhang, D., Lai, C., Zhang, S., Ma, J., Wei, Y., Yu, Q., Lv, W., Yu, Y., Li, B., Yang, Q.-H., Yang, Y., Lu, J., & Kang, F. (2019). Cross-linked beta alumina nanowires with compact gel polymer electrolyte coating for ultra-stable sodium metal battery. Nature Communications. https://doi.org/10.1038/s41467-019-11960-w
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