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Efficient electrochemical production of glucaric acid and H2 via glucose electrolysis
Open accessAbstract
Glucose electrolysis offers a prospect of value-added glucaric acid synthesis and energy-saving hydrogen production from the biomass-based platform molecules. Here we report that nanostructured NiFe oxide (NiFeO x) and nitride (NiFeN x) catalysts, synthesized from NiFe layered double hydroxide nanosheet arrays on three-dimensional Ni foams, demonstrate a high activity and selectivity towards anodic glucose oxidation. The electrolytic cell assembled with these two catalysts can deliver 100 mA cm−2 at 1.39 V. A faradaic efficiency of 87% and glucaric acid yield of 83% are obtained from the glucose electrolysis, which takes place via a guluronic acid pathway evidenced by in-situ infrared spectroscopy. A rigorous process model combined with a techno-economic analysis shows that the electrochemical reduction of glucose produces glucaric acid at a 54% lower cost than the current chemical approach. This work suggests that glucose electrolysis is an energy-saving and cost-effective approach for H 2 production and biomass valorization.
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The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Hydroxymethylfurfural, A Versatile Platform Chemical Made from Renewable Resources
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Conversion of Biomass into Chemicals over Metal Catalysts
Besson, M., Gallezot, P., & Pinel, C. (2014) · Chemical Reviews · doi:10.1021/cr4002269 · Cited by 1,780
Zhang, B., Xiao, C., Xie, S., Liang, J., Chen, X., & Tang, Y. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b02610 · Cited by 509
Wang, T., Nam, G., Jin, Y., Wang, X., Ren, P., Kim, M. G., Liang, J., Wen, X., Jang, H., Han, J., et al. (2018) · Advanced Materials · doi:10.1002/adma.201800757 · Cited by 318
Cited by
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Catalytic conversion of lignocellulosic biomass into chemicals and fuels
Deng, W., Feng, Y., Fu, J., Guo, H., Guo, Y., Han, B., Jiang, Z., Kong, L., Li, C., Liu, H., et al. (2023) · Green Energy & Environment · doi:10.1016/j.gee.2022.07.003 · Cited by 854
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Qi, Y., Zhang, Y., Yang, L., Zhao, Y., Zhu, Y., Jiang, H., & Li, C. (2022) · Nature Communications · doi:10.1038/s41467-022-32443-5 · Cited by 490
Han, X., Sheng, H., Yu, C., Walker, T. W., Huber, G. W., Qiu, J., & Jin, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01498 · Cited by 445
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Metadata
- Authors
- Liu, W.-J., Xu, Z., Zhao, D., Pan, X.-Q., Li, H.-C., Hu, X., Fan, Z.-Y., Wang, W.-K., Zhao, G.-H., Jin, S., Huber, G. W., & Yu, H.-Q.
- Venue
- Nature Communications
- Published
- 2020-01-14
- Volume
- 11
- Issue
- 1
- Pages
- 265-265
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2999372363
- Cited by
- 612
- References
- 5
- FWCI
- 22.12
- Type
- journal article
- Language
- en
- Open access
- gold
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- Liu, W.-J., Xu, Z., Zhao, D., Pan, X.-Q., Li, H.-C., Hu, X., Fan, Z.-Y., Wang, W.-K., Zhao, G.-H., Jin, S., Huber, G. W., & Yu, H.-Q. (2020). Efficient electrochemical production of glucaric acid and H2 via glucose electrolysis. Nature Communications. https://doi.org/10.1038/s41467-019-14157-3
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