Ultrafast terahertz magnetometry
Open accessAbstract
A material’s magnetic state and its dynamics are of great fundamental research interest and are also at the core of a wide plethora of modern technologies. However, reliable access to magnetization dynamics in materials and devices on the technologically relevant ultrafast timescale, and under realistic device-operation conditions, remains a challenge. Here, we demonstrate a method of ultrafast terahertz (THz) magnetometry, which gives direct access to the (sub-)picosecond magnetization dynamics even in encapsulated materials or devices in a contact-free fashion, in a fully calibrated manner, and under ambient conditions. As a showcase for this powerful method, we measure the ultrafast magnetization dynamics in a laser-excited encapsulated iron film. Our measurements reveal and disentangle distinct contributions originating from (i) incoherent hot-magnon-driven magnetization quenching and (ii) coherent acoustically-driven modulation of the exchange interaction in iron, paving the way to technologies utilizing ultrafast heat-free control of magnetism. High sensitivity and relative ease of experimental arrangement highlight the promise of ultrafast THz magnetometry for both fundamental studies and the technological applications of magnetism.
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THz emission spectroscopy has emerged as a potentially valuable contact-free probe of magnetization dynamics in a variety of materials.
“THz emission spectroscopy has emerged as a potentially valuable contact-free probe of magnetization dynamics in a variety of materials122.”
From Ultrafast terahertz emission from emerging symmetry-broken materials (2023) · cites this paper as [122]
When a thin FM metallic film is combined with a non-magnetic layer in a heterostructure, the THz emission intensity is dramatically enhanced far beyond what is expected from demagnetization in the magnetic layer alone.
“when a thin FM metallic film is combined with a non-magnetic (NM) layer in a heterostructure configuration, the THz emission intensity is dramatically enhanced, far beyond what is expected from demagnetization in the magnetic layer alone53,122.”
From Ultrafast terahertz emission from emerging symmetry-broken materials (2023) · cites this paper as [122]
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Quantitative Terahertz Magnetometry
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Terahertz wave radiation simulation in the Fe thin film*
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- Authors
- Zhang, W., Maldonado, P., Jin, Z., Seifert, T. S., Arabski, J., Schmerber, G., Beaurepaire, E., Bonn, M., Kampfrath, T., Oppeneer, P. M., & Turchinovich, D.
- Affiliations
- Bielefeld University (DE)
- Uppsala University (SE)
- University of Shanghai for Science and Technology (CN)
- ETH Zurich (CH)
- Centre National de la Recherche Scientifique (FR)
- Max Planck Institute for Polymer Research (DE)
- Freie Universität Berlin (DE)
- Corresponding author
- Turchinovich, Dmitry
- ORCID
- Venue
- Nature Communications
- Published
- 2020-08-25
- Volume
- 11
- Issue
- 1
- Pages
- 4247-4247
- ISSN
- 2041-1723 (ISSN-L)
- PMC
- PMC7447779
- OpenAlex
- W3080725279
- Cited by
- 110
- References
- 61
- Citations by year
- 2026: 7 · 2025: 21 · 2024: 15 · 2023: 27 · 2022: 22 · 2021: 17 · 2020: 1
- FWCI
- 6.76
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nature Communications (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- Refubium (Universitätsbibliothek der Freien Universität Berlin) (submittedVersion, cc-by)
- Uppsala University Publications (Uppsala University) (submittedVersion, other-oa)
- HAL (submittedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Publikationen an der Universität Bielefeld (Universität Bielefeld) (submittedVersion, cc-by)
- MPG.PuRe (Max Planck Society) (submittedVersion, other-oa)
- Repository for Publications and Research Data (ETH Zurich) (submittedVersion, cc-by)
- Universitätsbibliothek der FU Berlin Hochschulschriftenstelle u. Dokumentenserver (cc-by)
- ETH Zürich Research Collection (cc-by)
- Funders
- Chinese Scholarship Council
- Vetenskapsrådet
- Knut och Alice Wallenbergs Stiftelse (2015.0060)
- Swedish National Infrastructure for Computing
- Deutsche Forschungsgemeinschaft (278162697 – SFB 1242)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Magnetic properties of thin films
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Advanced Condensed Matter Physics
- Keywords
- magnetization dynamics, iron films, non-contact measurement
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