The DOI matches its Crossref record; 55 of the 55 references it cites were found in a registry or an index.
Highly active and selective oxygen reduction to H2O2 on boron-doped carbon for high production rates
Open accessAbstract
Oxygen reduction reaction towards hydrogen peroxide (H 2 O 2) provides a green alternative route for H 2 O 2 production, but it lacks efficient catalysts to achieve high selectivity and activity simultaneously under industrial-relevant production rates. Here we report a boron-doped carbon (B-C) catalyst which can overcome this activity-selectivity dilemma. Compared to the state-of-the-art oxidized carbon catalyst, B-C catalyst presents enhanced activity (saving more than 210 mV overpotential) under industrial-relevant currents (up to 300 mA cm−2) while maintaining high H 2 O 2 selectivity (85–90%). Density-functional theory calculations reveal that the boron dopant site is responsible for high H 2 O 2 activity and selectivity due to low thermodynamic and kinetic barriers. Employed in our porous solid electrolyte reactor, the B-C catalyst demonstrates a direct and continuous generation of pure H 2 O 2 solutions with high selectivity (up to 95%) and high H 2 O 2 partial currents (up to ~400 mA cm−2), illustrating the catalyst’s great potential for practical applications in the future.
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Double-slit photoelectron interference in strong-field ionization of the neon dimer
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Self-citationImproved Oxygen Reduction Activity on Pt 3 Ni(111) via Increased Surface Site Availability
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High-efficiency oxygen reduction to hydrogen peroxide catalysed by oxidized carbon materials
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Self-citationEnabling direct H2O2 production through rational electrocatalyst design
Siahrostami, S., Verdaguer-Casadevall, A., Karamad, M., Deiana, D., Malacrida, P., Wickman, B., Escudero-Escribano, M., Paoli, E. A., Frydendal, R., Hansen, T. W., et al. (2013) · Nature Materials · doi:10.1038/nmat3795 · Cited by 1,597
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Cited by
Cation‐Vacancy‐Enriched Nickel Phosphide for Efficient Electrosynthesis of Hydrogen Peroxides
Zhou, Z., Kong, Y., Tan, H., Huang, Q., Wang, C., Pei, Z., Wang, H., Liu, Y., Wang, Y., Li, S., et al. (2022) · Advanced Materials · doi:10.1002/adma.202106541 · Cited by 325
Self-citationAhmadi, M., Adeleye, O., Vonalt, G., & Nazemi, M. (2025) · Environmental Science & Technology · doi:10.1021/acs.est.5c04748 · Cited by 41
Metadata
- Authors
- Xia, Y., Zhao, X., Xia, C., Wu, Z.-Y., Zhu, P., Kim, J. Y., Bai, X., Gao, G., Hu, Y., Zhong, J., Liu, Y., & Wang, H.
- Venue
- Nature Communications
- Published
- 2021-07-09
- Volume
- 12
- Issue
- 1
- Pages
- 4225-4225
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3178877678
- Cited by
- 499
- References
- 55
- FWCI
- 14.46
- Type
- journal article
- Language
- en
- Open access
- gold
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- Xia, Y., Zhao, X., Xia, C., Wu, Z.-Y., Zhu, P., Kim, J. Y., Bai, X., Gao, G., Hu, Y., Zhong, J., Liu, Y., & Wang, H. (2021). Highly active and selective oxygen reduction to H2O2 on boron-doped carbon for high production rates. Nature Communications. https://doi.org/10.1038/s41467-021-24329-9
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