The DOI matches its Crossref record; 59 of the 59 references it cites were found in a registry or an index.
Nano-crumples induced Sn-Bi bimetallic interface pattern with moderate electron bank for highly efficient CO2 electroreduction
Open accessAbstract
CO 2 electroreduction reaction offers an attractive approach to global carbon neutrality. Industrial CO 2 electrolysis towards formate requires stepped-up current densities, which is limited by the difficulty of precisely reconciling the competing intermediates (COOH* and HCOO*). Herein, nano-crumples induced Sn-Bi bimetallic interface-rich materials are in situ designed by tailored electrodeposition under CO 2 electrolysis conditions, significantly expediting formate production. Compared with Sn-Bi bulk alloy and pure Sn, this Sn-Bi interface pattern delivers optimum upshift of Sn p-band center, accordingly the moderate valence electron depletion, which leads to weakened Sn-C hybridization of competing COOH* and suitable Sn-O hybridization of HCOO*. Superior partial current density up to 140 mA/cm 2 for formate is achieved. High Faradaic efficiency (>90%) is maintained at a wide potential window with a durability of 160 h. In this work, we elevate the interface design of highly active and stable materials for efficient CO 2 electroreduction.
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Self-citationAdvances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
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Interface-Engineered Cu/Cu2In Metallic Aerogels for Efficient Electrochemical CO2 Reduction
Chen, C., Huang, H., Chen, Y., Zhang, Z., Fu, H., Li, H., Huang, W.-H., Lai, F., Zhang, N., & Liu, T. (2024) · ACS Materials Letters · doi:10.1021/acsmaterialslett.3c01473 · Cited by 14
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Metadata
- Authors
- Ren, B., Wen, G., Gao, R., Luo, D., Zhang, Z., Qiu, W., Ma, Q., Wang, X., Cui, Y., Ricardez–Sandoval, L., Yu, A., & Chen, Z.
- Venue
- Nature Communications
- Published
- 2022-05-05
- Volume
- 13
- Issue
- 1
- Pages
- 2486-2486
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W4229029543
- Cited by
- 285
- References
- 59
- FWCI
- 10.74
- Type
- journal article
- Language
- en
- Open access
- gold
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- Ren, B., Wen, G., Gao, R., Luo, D., Zhang, Z., Qiu, W., Ma, Q., Wang, X., Cui, Y., Ricardez–Sandoval, L., Yu, A., & Chen, Z. (2022). Nano-crumples induced Sn-Bi bimetallic interface pattern with moderate electron bank for highly efficient CO2 electroreduction. Nature Communications. https://doi.org/10.1038/s41467-022-29861-w
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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