The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Dual interfacial engineering of a Chevrel phase electrode material for stable hydrogen evolution at 2500 mA cm−2
Open accessAbstract
Constructing stable electrodes which function over long timescales at large current density is essential for the industrial realization and implementation of water electrolysis. However, rapid gas bubble detachment at large current density usually results in peeling-off of electrocatalysts and performance degradation, especially for long term operations. Here we construct a mechanically-stable, all-metal, and highly active CuMo 6 S 8/Cu electrode by in-situ reaction between MoS 2 and Cu. The Chevrel phase electrode exhibits strong binding at the electrocatalyst-support interface with weak adhesion at electrocatalyst-bubble interface, in addition to fast hydrogen evolution and charge transfer kinetics. These features facilitate the achievement of large current density of 2500 mA cm−2 at a small overpotential of 334 mV which operate stably at 2500 mA cm−2 for over 100 h. In-situ total internal reflection imaging at micrometer level and mechanical tests disclose the relationships of two interfacial forces and performance of electrocatalysts. This dual interfacial engineering strategy can be extended to construct stable and high-performance electrodes for other gas-involving reactions.
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Cites
Double-slit photoelectron interference in strong-field ionization of the neon dimer
Kunitski, M., Eicke, N., Huber, P., Köhler, J., Zeller, S., Voigtsberger, J., Schlott, N., Henrichs, K., Sann, H., Trinter, F., et al. (2019) · Nature Communications · doi:10.1038/s41467-018-07882-8 · Cited by 8,162
Structural absorption by barbule microstructures of super black bird of paradise feathers
McCoy, D. E., Feo, T., Harvey, T. A., & Prum, R. O. (2018) · Nature Communications · doi:10.1038/s41467-017-02088-w · Cited by 7,424
Ultrastrong adhesion of graphene membranes
Koenig, S. P., Boddeti, N. G., Dunn, M. L., & Bunch, J. S. (2011) · Nature Nanotechnology · doi:10.1038/nnano.2011.123 · Cited by 1,107
Han, N., Yang, K. R., Lu, Z., Li, Y., Xu, W., Gao, T., Cai, Z., Zhang, Y., Batista, V. S., Liu, W., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-03429-z · Cited by 766
Luo, Y., Tang, L., Khan, U., Yu, Q., Cheng, H.-M., Zou, X., & Liu, B. (2019) · Nature Communications · doi:10.1038/s41467-018-07792-9 · Cited by 713
Self-citationSuperwetting Electrodes for Gas-Involving Electrocatalysis
Xu, W., Lu, Z., Sun, X., Jiang, L., & Duan, X. (2018) · Accounts of Chemical Research · doi:10.1021/acs.accounts.8b00070 · Cited by 638
Cited by
Wan, L., Xu, Z., Xu, Q., Pang, M., Lin, D., Liu, J., & Wang, B. (2023) · Energy & Environmental Science · doi:10.1039/d3ee00142c · Cited by 371
Bubble Engineering on Micro-/Nanostructured Electrodes for Water Splitting
Li, M., Xie, P., Yu, L., Luo, L., & Sun, X. (2023) · ACS Nano · doi:10.1021/acsnano.3c08831 · Cited by 286
Yao, R., Sun, K., Zhang, K., Wu, Y., Du, Y., Zhao, Q., Liu, G., Chen, C., Sun, Y., & Li, J. (2024) · Nature Communications · doi:10.1038/s41467-024-46553-9 · Cited by 262
Unlocking Efficiency: Minimizing Energy Loss in Electrocatalysts for Water Splitting
Li, W., Liu, Y., Azam, A., Liu, Y., Yang, J., Wang, D., Sorrell, C. C., Zhao, C., & Li, S. (2024) · Advanced Materials · doi:10.1002/adma.202404658 · Cited by 162
Self-citationWang, J., Liang, C., Ma, X., Liu, P., Pan, W., Zhu, H., Guo, Z., Sui, Y., Liu, H., Liu, L., et al. (2024) · Advanced Materials · doi:10.1002/adma.202307925 · Cited by 124
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Metadata
- Authors
- Liu, H., Xie, R., Luo, Y., Cui, Z., Yu, Q., Gao, Z., Zhang, Z., Yang, F., Kang, X., Ge, S., Li, S., Gao, X., Chai, G., Liu, L., & Liu, B.
- Venue
- Nature Communications
- Published
- 2022-10-26
- Volume
- 13
- Issue
- 1
- Pages
- 6382-6382
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W4307313886
- Cited by
- 230
- References
- 6
- FWCI
- 8.55
- Type
- journal article
- Language
- en
- Open access
- gold
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- Liu, H., Xie, R., Luo, Y., Cui, Z., Yu, Q., Gao, Z., Zhang, Z., Yang, F., Kang, X., Ge, S., Li, S., Gao, X., Chai, G., Liu, L., & Liu, B. (2022). Dual interfacial engineering of a Chevrel phase electrode material for stable hydrogen evolution at 2500 mA cm−2. Nature Communications. https://doi.org/10.1038/s41467-022-34121-y
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