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The DOI matches its Crossref record; 42 of the 42 references it cites were found in a registry or an index.

Ultraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management

Open access
Jing, Yaoge, Zhao, Zhengchuang, Cao, Xiaoling, Sun, Qinrong, Yuan, Yanping, Li, Tingxian·2023·Nature Communications

Abstract

Phase change materials (PCMs) offer great potential for realizing zero-energy thermal management due to superior thermal storage and stable phase-change temperatures. However, liquid leakage and solid rigidity of PCMs are long-standing challenges for PCM-based wearable thermal regulation. Here, we report a facile and cost-effective chemical cross-linking strategy to develop ultraflexible polymer-based phase change composites with a dual 3D crosslinked network of olefin block copolymers (OBC) and styrene-ethylene-butylene-styrene (SEBS) in paraffin wax (PW). The C-C bond-enhanced OBC-SEBS networks synergistically improve the mechanical, thermal, and leakage-proof properties of PW@OBC-SEBS. Notably, the proposed peroxide-initiated chemical cross-linking method overcomes the limitations of conventional physical blending methods and thus can be applicable across diverse polymer matrices. We further demonstrate a portable and flexible PW@OBC-SEBS module that maintains a comfortable temperature range of 39–42 °C for personal thermotherapy. Our work provides a promising route to fabricate scalable polymer-based phase change composite for wearable thermal management.

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Metadata

Authors
Jing, Y., Zhao, Z., Cao, X., Sun, Q., Yuan, Y., & Li, T.
Venue
Nature Communications
Published
2023-12-05
Volume
14
Issue
1
Pages
8060-8060
ISSN
2041-1723 (ISSN-L)
OpenAlex
W4389330830
Cited by
259
References
42
FWCI
25.37
Type
journal article
Language
en
Open access
gold

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CoChat. (2026). Citation check: Ultraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management. https://app.cochat.ai/papers/10.1038/s41467-023-43772-4
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Jing, Y., Zhao, Z., Cao, X., Sun, Q., Yuan, Y., & Li, T. (2023). Ultraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management. Nature Communications. https://doi.org/10.1038/s41467-023-43772-4

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