The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Glassy Li metal anode for high-performance rechargeable Li batteries
Open accessAbstract
Lithium metal has been considered an ideal anode for high-energy rechargeable Li batteries, although its nucleation and growth process remains mysterious, especially at the nanoscale. Here, cryogenic transmission electron microscopy was used to reveal the evolving nanostructure of Li metal deposits at various transient states in the nucleation and growth process, in which a disorder–order phase transition was observed as a function of current density and deposition time. The atomic interaction over wide spatial and temporal scales was depicted by reactive molecular dynamics simulations to assist in understanding the kinetics. Compared to crystalline Li, glassy Li outperforms in electrochemical reversibility, and it has a desired structure for high-energy rechargeable Li batteries. Our findings correlate the crystallinity of the nuclei with the subsequent growth of the nanostructure and morphology, and provide strategies to control and shape the mesostructure of Li metal to achieve high performance in rechargeable Li batteries. Lithium metal is considered an ideal anode for high-energy rechargeable lithium batteries, but understanding its nucleation and growth at the nanoscale remains challenging. Using cryogenic transmission electron microscopy and simulations, a structural and morphological evolution scenario for Li deposits is proposed.
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Cites
Atomic structure of sensitive battery materials and interfaces revealed by cryo–electron microscopy
Li, Y., Li, Y., Pei, A., Yan, K., Sun, Y., Wu, C.-L., Joubert, L.-M., Chin, R., Koh, A. L., Yu, Y., et al. (2017) · Science · doi:10.1126/science.aam6014 · Cited by 1,547
Self-citationA Review of Classical and Nonclassical Nucleation Theories
Karthika, S., Radhakrishnan, T. K., & Kalaichelvi, P. (2016) · Crystal Growth & Design · doi:10.1021/acs.cgd.6b00794 · Cited by 868
Wang, X., Zhang, M., Alvarado, J., Wang, S., Sina, M., Lu, B., Bouwer, J., Xu, W., Xiao, J., Zhang, J.-G., et al. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b03606 · Cited by 409
Self-citationOrsini, F., Du Pasquier, A., Beaudoin, B., Tarascon, J. M., Trentin, M., Langenhuizen, N., De Beer, E., & Notten, P. (1998) · Journal of Power Sources · doi:10.1016/s0378-7753(98)00128-1 · Cited by 310
Cited by
Han, B., Zhang, Z., Zou, Y., Xu, K., Xu, G., Wang, H., Meng, H., Deng, Y., Li, J., & Gu, M. (2021) · Advanced Materials · doi:10.1002/adma.202100404 · Cited by 346
Strategies towards enabling lithium metal in batteries: interphases and electrodes
Horstmann, B., Shi, J., Amine, R., Werres, M., He, X., Jia, H., Hausen, F., Cekic-Laskovic, I., Wiemers-Meyer, S., Lopez, J., et al. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00767j · Cited by 298
Insights into the deposition chemistry of Li ions in nonaqueous electrolyte for stable Li anodes
Wang, Z., Sun, Z., Li, J., Shi, Y., Sun, C., An, B., Cheng, H.-M., & Li, F. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01017k · Cited by 268
Metadata
- Authors
- Wang, X., Pawar, G., Li, Y., Ren, X., Zhang, M., Lu, B., Banerjee, A., Liu, P., Dufek, E. J., Zhang, J.-G., Xiao, J., Liu, J., Meng, Y. S., & Liaw, B.
- Venue
- Nature Materials
- Published
- 2020-07-27
- Volume
- 19
- Issue
- 12
- Pages
- 1339-1345
- ISSN
- 1476-1122 (ISSN-L)
- 1476-4660
- OpenAlex
- W2981565008
- Cited by
- 269
- References
- 4
- FWCI
- 13.67
- Type
- journal article
- Language
- en
- Open access
- green
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- Wang, X., Pawar, G., Li, Y., Ren, X., Zhang, M., Lu, B., Banerjee, A., Liu, P., Dufek, E. J., Zhang, J.-G., Xiao, J., Liu, J., Meng, Y. S., & Liaw, B. (2020). Glassy Li metal anode for high-performance rechargeable Li batteries. Nature Materials. https://doi.org/10.1038/s41563-020-0729-1
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