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Cited by 220

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High-harmonic generation from an epsilon-near-zero material

Open access
Yang, Yuanmu, Lu, Jian, Manjavacas, Alejandro, Luk, Ting S., Liu, Hanzhe, Kelley, Kyle, Maria, Jon-Paul, Runnerstrom, Evan L., Sinclair, Michael B., Ghimire, Shambhu, Brener, Igal·2019·Nature Physics

Abstract

High-harmonic generation (HHG) is a signature optical phenomenon of strongly driven, nonlinear optical systems. Specifically, the understanding of the HHG process in rare gases has played a key role in the development of attosecond science1. Recently, HHG has also been reported in solids, providing novel opportunities such as controlling strong-field and attosecond processes in dense optical media down to the nanoscale2. Here, we report HHG from a low-loss, indium-doped cadmium oxide thin film by leveraging the epsilon-near-zero (ENZ) effect3–8, whereby the real part of the material’s permittivity in certain spectral ranges vanishes, as well as the associated large resonant enhancement of the driving laser field. We find that ENZ-assisted harmonics exhibit a pronounced spectral redshift as well as linewidth broadening, resulting from the photo induced electron heating and the consequent time-dependent ENZ wavelength of the material. Our results provide a new platform to study strong-field and ultrafast electron dynamics in ENZ materials, reveal new degrees of freedom for spectral and temporal control of HHG, and open up the possibilities of compact solid-state attosecond light sources.High harmonics are generated from a thin film by leveraging the epsilon-near-zero effect. These kinds of harmonic are found to exhibit a pronounced spectral redshift as well as linewidth broadening caused by the time-dependency of this effect.

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Metadata

Authors
Yang, Y., Lu, J., Manjavacas, A., Luk, T. S., Liu, H., Kelley, K., Maria, J.-P., Runnerstrom, E. L., Sinclair, M. B., Ghimire, S., & Brener, I.
Venue
Nature Physics
Published
2019-07-15
Volume
15
Issue
10
Pages
1022-1026
ISSN
  • 1745-2473 (ISSN-L)
  • 1745-2481
OpenAlex
W2956847291
Cited by
220
References
2
FWCI
10.33
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: High-harmonic generation from an epsilon-near-zero material. https://app.cochat.ai/papers/10.1038/s41567-019-0584-7
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Yang, Y., Lu, J., Manjavacas, A., Luk, T. S., Liu, H., Kelley, K., Maria, J.-P., Runnerstrom, E. L., Sinclair, M. B., Ghimire, S., & Brener, I. (2019). High-harmonic generation from an epsilon-near-zero material. Nature Physics. https://doi.org/10.1038/s41567-019-0584-7

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