Multi-functional 2D hybrid aerogels for gas absorption applications
Open accessAbstract
Aerogels have attracted significant attention recently due to their ultra-light weight porous structure, mechanical robustness, high electrical conductivity, facile scalability and their use as gas and oil absorbers. Herein, we examine the multi-functional properties of hybrid aerogels consisting of reduced graphene oxide (rGO) integrated with hexagonal boron nitride (hBN) platelets. Using a freeze-drying approach, hybrid aerogels are fabricated by simple mixing with various volume fractions of hBN and rGO up to 0.5/0.5 ratio. The fabrication method is simple, cost effective, scalable and can be extended to other 2D materials combinations. The hybrid rGO/hBN aerogels (HAs) are mechanically robust and highly compressible with mechanical properties similar to those of the pure rGO aerogel. We show that the presence of hBN in the HAs enhances the gas absorption capacities of formaldehyde and water vapour up to ~ 7 and > 8 times, respectively, as compared to pure rGO aerogel. Moreover, the samples show good recoverability, making them highly efficient materials for gas absorption applications and for the protection of artefacts such as paintings in storage facilities. Finally, even in the presence of large quantity of insulating hBN, the HAs are electrically conductive, extending the potential application spectrum of the proposed hybrids to the field of electro-thermal actuators. The work proposed here paves the way for the design and production of novel 2D materials combinations with tailored multi-functionalities suited for a large variety of modern applications.
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Raman spectra of NCSe@GA and NCSe@MGA show three additional peaks at ~1369, ~1575, and ~2601 cm−1 representing D-band, G-band, and 2D(G*)-band from rGO contents.
“Raman spectra of NCSe@GA and NCSe@MGA showed three additional peaks at ~1369, ~1575 and ~2601 cm− 1 representing typical D-band, G-band and 2D(G*)-band from rGO contents [71].”
From Rationally designed multifunctional Ti3C2 MXene@Graphene composite aerogel integrated with bimetallic selenides for enhanced supercapacitor performance and overall water splitting (2022) · cites this paper as [71]
The Results and discussion section (Fig. 3; page not provided) identifies characteristic D and G Raman peaks in rGO aerogels, supporting that part of the band assignment. It does not report spectra for NCSe@GA or NCSe@MGA, the claimed peak positions (~1369, ~1575, and ~2601 cm−1), or a 2D(G*) peak. (LLM, conf=0.88)
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Self-citation
- Authors
- Androulidakis, C., Kotsidi, M., Gorgolis, G., Pavlou, C., Sygellou, L., Paterakis, G., Koutroumanis, N., & Galiotis, C.
- Affiliations
- Foundation for Research and Technology Hellas (GR)
- University of Patras (GR)
- Corresponding author
- Galiotis, Costas
- ORCID
- Pavlou, Christos
- Venue
- Scientific Reports
- Published
- 2021-06-30
- Volume
- 11
- Issue
- 1
- Pages
- 13548-13548
- ISSN
- 2045-2322 (ISSN-L)
- PMC
- PMC8245581
- OpenAlex
- W3173228770
- Cited by
- 30
- References
- 57
- Citations by year
- 2026: 10 · 2025: 4 · 2024: 7 · 2023: 3 · 2022: 6
- FWCI
- 1.46
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Scientific Reports (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- arXiv (Cornell University) (cc-by)
- Funders
- University of Patras
- Graphene Flagship (881603)
- General Secretariat for Research and Technology
- Topics
- Physical Sciences › Chemistry › Spectroscopy › Aerogels and thermal insulation
- Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Keywords
- hybrid aerogels, reduced graphene oxide, hexagonal boron nitride, gas absorption, formaldehyde adsorption, water vapor adsorption, freeze-drying, mechanical robustness, electrical conductivity, electrothermal actuator, two-dimensional materials
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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