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Honeycomb structured porous films prepared from carbohydrate based polymers synthesized via the RAFT process
Abstract
Carbohydrate based polystyrene was synthesized via RAFT polymerization. The RAFT agents were based on α-D-glucose, β-cyclodextrin and modified cellulose to obtain polystyrene with a polar head or polystyrene with a star or comb structure, respectively. The polymerizations were carried out in different solvents. The molecular weight of the linear polymer was found to develop according to the expected values, but the synthesis of the carbohydrate based polymers was influenced by other parameters. The molecular weight for the star polymer synthesis showed a pronounced deviation due to the reduced accessibility of the RAFT group at higher conversions of the polymerization. Films of these carbohydrate containing polystyrenes were cast from carbon disulfide and dichloromethane producing highly regular honeycomb structured films with pore diameters between 0.5 and 4 µm. The pore size was influenced by the polymers used as well as by the casting conditions.
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Cites
Chong, ). Y. K., Le, T. P. T., Moad, G., Rizzardo, E., & Thang, S. H. (1999) · Macromolecules · doi:10.1021/ma981472p · Cited by 850
Cited by
Bioapplications of RAFT Polymerization
Boyer, C., Bulmus, V., Davis, T. P., Ladmiral, V., Liu, J., & Perrier, S. (2009) · Chemical Reviews · doi:10.1021/cr9001403 · Cited by 1,015
Self-citationBiopolymer-based microgels/nanogels for drug delivery applications
Oh, J. K., Lee, D. I., & Park, J. M. (2009) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2009.08.001 · Cited by 542
Gregory, A., & Stenzel, M. H. (2012) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2011.08.004 · Cited by 470
Self-citationFavier, A., & Charreyre, M. (2006) · Macromolecular Rapid Communications · doi:10.1002/marc.200500839 · Cited by 461
Telechelic polymers by living and controlled/living polymerization methods
Tasdelen, M. A., Kahveci, M. U., & Yagci, Y. (2011) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2010.10.002 · Cited by 393
Metadata
- Authors
- Stenzel, M. H., Davis, T. P., & Fane, A. G.
- Venue
- Journal of Materials Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2003
- Volume
- 13
- Issue
- 9
- Pages
- 2090
- ISSN
- 0959-9428 (ISSN-L)
- 1364-5501
- OpenAlex
- W2158293205
- Cited by
- 207
- References
- 1
- FWCI
- 8.69
- Type
- journal article
- Language
- en
- Open access
- closed
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- Stenzel, M. H., Davis, T. P., & Fane, A. G. (2003). Honeycomb structured porous films prepared from carbohydrate based polymers synthesized via the RAFT process. Journal of Materials Chemistry. https://doi.org/10.1039/b304204a
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
