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Copper dioxygen (bio)inorganic chemistry
Open accessAbstract
Cu/O2 intermediates in biological, homogeneous, and heterogeneous catalysts exhibit unique spectral features that reflect novel geometric and electronic structures that make significant contributions to reactivity. This review considers how the respective intermediate electronic structures overcome the spin-forbidden nature of O2 binding, activate O2 for electrophilic aromatic attack and H-atom abstraction, catalyze the 4 e- reduction of O2 to H2O, and discusses the role of exchange coupling between Cu ions in determining reactivity.
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Citations
Cites
Multicopper oxidases and oxygenases
Solomon, E. I., Sundaram, U. M., & Machonkin, T. E. (1996) · Chemical Reviews · doi:10.1021/cr950046o · Cited by 3,664
Self-citation
Cited by
Copper Active Sites in Biology
Solomon, E. I., Heppner, D. E., Johnston, E. M., Ginsbach, J. W., Cirera, J., Qayyum, M., Kieber-Emmons, M. T., Kjaergaard, C. H., Hadt, R. G., & Tian, L. (2014) · Chemical Reviews · doi:10.1021/cr400327t · Cited by 1,751
Self-citationMetabolism and functions of copper in brain
Scheiber, I. F., Mercer, J. F. B., & Dringen, R. (2014) · Progress in Neurobiology · doi:10.1016/j.pneurobio.2014.01.002 · Cited by 506
Bioinspired Metal–Organic Framework Catalysts for Selective Methane Oxidation to Methanol
Baek, J., Rungtaweevoranit, B., Pei, X., Park, M., Fakra, S. C., Liu, Y.-S., Matheu, R., Alshmimri, S. A., Alshehri, S., Trickett, C. A., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b11525 · Cited by 417
Enzymatic Oxidation of Methane
Sirajuddin, S., & Rosenzweig, A. C. (2015) · Biochemistry · doi:10.1021/acs.biochem.5b00198 · Cited by 342
Oxidation Reactions with Bioinspired Mononuclear Non‐Heme Metal–Oxo Complexes
Engelmann, X., Monte‐Pérez, I., & Ray, K. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201600507 · Cited by 300
Metadata
- Authors
- Solomon, E. I., Ginsbach, J. W., Heppner, D. E., Kieber-Emmons, M. T., Kjaergaard, C. H., Smeets, P. J., Tian, L., & Woertink, J. S.
- Venue
- Faraday Discuss.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 148
- Pages
- 11-39
- ISSN
- 1359-6640 (ISSN-L)
- 1364-5498
- OpenAlex
- W2058949520
- Cited by
- 174
- References
- 1
- FWCI
- 9.32
- Type
- journal article
- Language
- en
- Open access
- green
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