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Dynamics of photogenerated holes in nanocrystalline α-Fe2O3electrodes for water oxidation probed by transient absorption spectroscopy
Open accessAbstract
Transient absorption spectroscopy on the μs-s time scale is used to monitor the yield and decay dynamics of photogenerated holes in nanocrystalline hematite photoanodes. In the absence of a positive applied bias, these holes are observed to undergo rapid electron-hole recombination. The application of a positive bias results in the generation of long-lived (3 ± 1 s lifetime) photoholes.
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Cites
Reduction potentials of one-electron couples involving free radicals in aqueous solution
Wardman, P. (1989) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555843 · Cited by 2,123
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
Cited by
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Moniz, S. J. A., Shevlin, S. A., Martin, D. J., Guo, Z.-X., & Tang, J. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03271c · Cited by 2,363
Self-citationTime-resolved observations of water oxidation intermediates on a cobalt oxide nanoparticle catalyst
Zhang, M., de Respinis, M., & Frei, H. (2014) · Nature Chemistry · doi:10.1038/nchem.1874 · Cited by 855
Barroso, M., Cowan, A. J., Pendlebury, S. R., Grätzel, M., Klug, D. R., & Durrant, J. R. (2011) · Journal of the American Chemical Society · doi:10.1021/ja205325v · Cited by 579
Self-citationHematite-based solar water splitting: challenges and opportunities
Lin, Y., Yuan, G., Sheehan, S., Zhou, S., & Wang, D. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01850g · Cited by 417
Metadata
- Authors
- Pendlebury, S. R., Barroso, M., Cowan, A. J., Sivula, K., Tang, J., Grätzel, M., Klug, D., & Durrant, J. R.
- Venue
- Chem. Commun.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 47
- Issue
- 2
- Pages
- 716-718
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W1971521588
- Cited by
- 281
- References
- 2
- FWCI
- 8.89
- Type
- journal article
- Language
- en
- Open access
- green
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- Pendlebury, S. R., Barroso, M., Cowan, A. J., Sivula, K., Tang, J., Grätzel, M., Klug, D., & Durrant, J. R. (2011). Dynamics of photogenerated holes in nanocrystalline α-Fe2O3electrodes for water oxidation probed by transient absorption spectroscopy. Chem. Commun. https://doi.org/10.1039/c0cc03627g
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