Reduction potentials of one-electron couples involving free radicals in aqueous solution
Abstract
Reduction of an electron acceptor (oxidant), A, or oxidation of an electron donor (reductant), A2−, is often achieved stepwise via one-electron processes involving the couples A/A⋅− or A⋅−/A2− (or corresponding prototropic conjugates such as A/AH⋅ or AH⋅/AH2). The intermediate A⋅−(AH⋅) is a free radical. The reduction potentials of such one-electron couples are of value in predicting the direction or feasibility, and in some instances the rate constants, of many free-radical reactions. Electrochemical methods have limited applicability in measuring these properties of frequently unstable species, but fast, kinetic spectrophotometry (especially pulse radiolysis) has widespread application in this area. Tables of ca. 1200 values of reduction potentials of ca. 700 one-electron couples in aqueous solution are presented. The majority of organic oxidants listed are quinones, nitroaryl and bipyridinium compounds. Reductants include phenols, aromatic amines, indoles and pyrimidines, thiols and phenothiazines. Inorganic couples largely involve compounds of oxygen, sulfur, nitrogen and the halogens. Proteins, enzymes and metals and their complexes are excluded.
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There are two standard redox potentials for O2•−: E′(O2/O2•−) = 0.33 V and E′(O2•−/H2O2) = 0.93 V.
“There are two standard redox potentials for O2•− showing that it can act as a reducing agent E′(O2/O2•−) = 0.33 V or as an oxidizing agent E′(O2•−/H2O2) = 0.93 V [15]), Figure 4.”
From Superoxide Anion Chemistry—Its Role at the Core of the Innate Immunity (2023) · cites this paper as [15]
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- Authors
- Wardman, P.
- Affiliations
- Mount Vernon Hospital (GB)
- Corresponding author
- Wardman, Peter
- ORCID
- Wardman, Peter
- Venue
- Journal of Physical and Chemical Reference Data
- Publisher
- AIP Publishing
- Published
- 1989-10-01
- Volume
- 18
- Issue
- 4
- Pages
- 1637-1755
- ISSN
- 0047-2689 (ISSN-L)
- 1529-7845
- OpenAlex
- W1979424160
- Cited by
- 2,123
- References
- 3
- Citations by year
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- FWCI
- 19.63
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Physical and Chemical Reference Data (publishedVersion)
- Topics
- Physical Sciences › Chemistry › Organic Chemistry › Free Radicals and Antioxidants
- Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Photochemistry and Electron Transfer Studies
- Keywords
- redox potential, free radicals, aqueous solutions, electron transfer, quinones, nitroaromatic compounds, phenols, aromatic amines, indole, pyrimidines, thiols, phenothiazines, inorganic oxidants, redox couples
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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