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Probing the surfaces of heterogeneous catalysts by in situ IR spectroscopy
Open accessAbstract
This critical review describes the reactivity of heterogeneous catalysts from the point of view of four simple, but essential for Chemistry, molecules (namely dihydrogen, carbon monoxide, nitrogen monoxide and ethylene) that are considered as probes or as reactants in combination with "in situ" controlled temperature and pressure Infrared spectroscopy. The fundamental properties of H(2), CO, NO and C(2)H(4) are shortly described in order to justify their different behaviour in respect of isolated sites in different environments, extended surfaces, clusters, crystalline or amorphous materials. The description is given by considering some "key studies" and trying to evidence similarities and differences among surfaces and probes (572 references).
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Cites
Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Photochemistry on Metal Nanoparticles
Watanabe, K., Menzel, D., Nilius, N., & Freund, H.-J. (2006) · Chemical Reviews · doi:10.1021/cr050167g · Cited by 486
Cited by
Valenzano, L., Civalleri, B., Chavan, S., Bordiga, S., Nilsen, M. H., Jakobsen, S., Lillerud, K. P., & Lamberti, C. (2011) · Chemistry of Materials · doi:10.1021/cm1022882 · Cited by 1,919
Self-citationCatalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Ouyang, M., Papanikolaou, K. G., Boubnov, A., Hoffman, A. S., Giannakakis, G., Bare, S. R., Stamatakis, M., Flytzani-Stephanopoulos, M., & Sykes, E. C. H. (2021) · Nature Communications · doi:10.1038/s41467-021-21555-z · Cited by 187
Ricci, M., Trewby, W., Cafolla, C., & Voïtchovsky, K. (2017) · Scientific Reports · doi:10.1038/srep43234 · Cited by 61
Metadata
- Authors
- Lamberti, C., Zecchina, A., Groppo, E., & Bordiga, S.
- Venue
- Chemical Society Reviews
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2010
- Volume
- 39
- Issue
- 12
- Pages
- 4951
- ISSN
- 0306-0012 (ISSN-L)
- 1460-4744
- OpenAlex
- W1998090485
- Cited by
- 491
- References
- 2
- FWCI
- 1.32
- Type
- journal article
- Language
- en
- Open access
- green
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- Lamberti, C., Zecchina, A., Groppo, E., & Bordiga, S. (2010). Probing the surfaces of heterogeneous catalysts by in situ IR spectroscopy. Chemical Society Reviews. https://doi.org/10.1039/c0cs00117a
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