Cited by 1,219Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceFuel Cells and Related Materials

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High oxygen-reduction activity and durability of nitrogen-doped graphene

Geng, Dongsheng, Chen, Ying, Chen, Yougui, Li, Yongliang, Li, Ruying, Sun, Xueliang, Ye, Siyu, Knights, Shanna·2011·Energy & Environmental Science

DOI 10.1039/c0ee00326c

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Abstract

Nitrogen-doped graphene as a metal-free catalyst for oxygen reduction was synthesized by heat-treatment of graphene using ammonia. It was found that the optimum temperature was 900 °C. The resulting catalyst had a very high oxygen reduction reaction (ORR) activity through a four-electron transfer process in oxygen-saturated 0.1 M KOH. Most importantly, the electrocatalytic activity and durability of this material are comparable or better than the commercial Pt/C (loading: 4.85 µgPt cm−2). XPS characterization of these catalysts was tested to identify the active N species for ORR.

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Authors: Geng, D., Chen, Y., Chen, Y., Li, Y., Li, R., Sun, X., Ye, S., & Knights, S.
Affiliations: Western University (CA)
Ballard Power Systems (Canada) (CA)
Corresponding author: Sun, Xueliang
ORCID: Geng, Dongsheng
Chen, Yougui
Li, Yongliang
Li, Ruying
Sun, Xueliang
Ye, Siyu
Venue: Energy & Environmental Science
Publisher: Royal Society of Chemistry (RSC)
Published: 2011
Volume: 4
Issue: 3
Pages: 760
ISSN: 1754-5692 (ISSN-L)
1754-5706
DOI: 10.1039/c0ee00326c
OpenAlex: W1999469559
Cited by: 1,219
References: 29
Citations by year: 2026: 10 · 2025: 23 · 2024: 34 · 2023: 26 · 2022: 47 · 2021: 53 · 2020: 71 · 2019: 121 · 2018: 132 · 2017: 133 · 2016: 132 · 2015: 147 · 2014: 122 · 2013: 94 · 2012: 60
FWCI: 38.58
Type: journal article
Language: en
Open access: closed
Locations: Energy & Environmental Science (publishedVersion)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Keywords: nitrogen-doped graphene, oxygen reduction reaction, metal-free electrocatalysts, ammonia treatment, heat treatment temperature, four-electron pathway, Pt/C comparison, alkaline electrolyte

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High oxygen-reduction activity and durability of nitrogen-doped graphene

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