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Small band gap copolymers based on furan and diketopyrrolopyrrole for field-effect transistors and photovoltaic cells
Open accessAbstract
Four small band gap semiconducting copolymers based on electron deficient diketopyrrolopyrrole alternating with electron rich trimers containing furan and benzene or thiophene have been synthesized via Suzuki polymerization. The polymers have optical band gaps between 1.4 and 1.6 eV, optimized for solar energy conversion, and exhibit ambipolar charge transport in field-effect transistors with hole and electron mobilities higher than 10−2 cm2 V−1 s−1. In solar cells the polymers are used as electron donors and provide power conversion efficiencies up to 3.7% in simulated solar light when mixed with [70]PCBM as acceptor.
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Cites
Umeyama, T., Takamatsu, T., Tezuka, N., Matano, Y., Araki, Y., Wada, T., Yoshikawa, O., Sagawa, T., Yoshikawa, S., & Imahori, H. (2009) · The Journal of Physical Chemistry C · doi:10.1021/jp902001z · Cited by 119
Cited by
Beaujuge, P. M., & Fréchet, J. M. J. (2011) · Journal of the American Chemical Society · doi:10.1021/ja2073643 · Cited by 1,427
Yiu, A. T., Beaujuge, P. M., Lee, O. P., Woo, C. H., Toney, M. F., & Fréchet, J. M. J. (2012) · Journal of the American Chemical Society · doi:10.1021/ja2089662 · Cited by 491
Ashraf, R. S., Meager, I., Nikolka, M., Kirkus, M., Planells, M., Schroeder, B. C., Holliday, S., Hurhangee, M., Nielsen, C. B., Sirringhaus, H., et al. (2015) · Journal of the American Chemical Society · doi:10.1021/ja511984q · Cited by 417
Advances in Charge Carrier Mobilities of Semiconducting Polymers Used in Organic Transistors
Holliday, S., Donaghey, J. E., & McCulloch, I. (2014) · Chemistry of Materials · doi:10.1021/cm402421p · Cited by 414
Diketopyrrolopyrroles: Synthesis, Reactivity, and Optical Properties
Grzybowski, M., & Gryko, D. T. (2015) · Advanced Optical Materials · doi:10.1002/adom.201400559 · Cited by 390
Metadata
- Authors
- Bijleveld, J. C., Karsten, B. P., Mathijssen, S. G. J., Wienk, M. M., de Leeuw, D. M., & Janssen, R. A. J.
- Venue
- J. Mater. Chem.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 21
- Issue
- 5
- Pages
- 1600-1606
- ISSN
- 0959-9428 (ISSN-L)
- 1364-5501
- OpenAlex
- W2097115769
- Cited by
- 160
- References
- 1
- FWCI
- 16.20
- Type
- journal article
- Language
- en
- Open access
- green
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- Bijleveld, J. C., Karsten, B. P., Mathijssen, S. G. J., Wienk, M. M., de Leeuw, D. M., & Janssen, R. A. J. (2011). Small band gap copolymers based on furan and diketopyrrolopyrrole for field-effect transistors and photovoltaic cells. J. Mater. Chem. https://doi.org/10.1039/c0jm03137b
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