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Role of photoactive layer morphology in high fill factor all-polymer bulk heterojunction solar cells
Open accessAbstract
We report on the realization of all-polymer solar cells based on blends of poly(3-hexylthiophene-2,5-diyl) (P3HT) as a donor and poly{[N,N′-bis(2-octyldodecyl)-naphthalene-1,4,5,8-bis(dicarboximide)-2,6-diyl]-alt-5,5′-(2,2′-bithiophene)} (P(NDI2OD-T2)) as an acceptor. High fill factors are demonstrated for the first time in this class of devices suggesting high dissociation efficiency for the bounded electron–hole pairs and balanced electron and hole mobility along the thin films. The use of the high-mobility n-type P(NDI2OD-T2) polymer enables us to overcome one of the problems limiting the efficiency of all-polymer solar cells, resulting in fill factors comparable with those reported for fullerene-based devices.
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Citations
Cited by
Polymer donor–polymer acceptor (all-polymer) solar cells
Facchetti, A. (2013) · Materials Today · doi:10.1016/j.mattod.2013.04.005 · Cited by 688
Self-citationSteyrleuthner, R., Schubert, M., Howard, I., Klaumünzer, B., Schilling, K., Chen, Z., Saalfrank, P., Laquai, F., Facchetti, A., & Neher, D. (2012) · Journal of the American Chemical Society · doi:10.1021/ja306844f · Cited by 458
Self-citationSynthesis and Photovoltaic Properties of New Metalloporphyrin-Containing Polyplatinyne Polymers
Zhan, H., Lamare, S., Ng, A., Kenny, T., Guernon, H., Chan, W.-K., Djurišić, A. B., Harvey, P. D., & Wong, W.-Y. (2011) · Macromolecules · doi:10.1021/ma2006206 · Cited by 127
Metadata
- Authors
- Fabiano, S., Chen, Z., Vahedi, S., Facchetti, A., Pignataro, B., & Loi, M. A.
- Venue
- Journal of Materials Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 21
- Issue
- 16
- Pages
- 5891
- ISSN
- 0959-9428 (ISSN-L)
- 1364-5501
- OpenAlex
- W2163539538
- Cited by
- 158
- References
- 0
- FWCI
- 13.37
- Type
- journal article
- Language
- en
- Open access
- green
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- Fabiano, S., Chen, Z., Vahedi, S., Facchetti, A., Pignataro, B., & Loi, M. A. (2011). Role of photoactive layer morphology in high fill factor all-polymer bulk heterojunction solar cells. Journal of Materials Chemistry. https://doi.org/10.1039/c0jm03405c
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