The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Tetrametallic molecular catalysts for photochemical water oxidation
Abstract
Among molecular water oxidation catalysts (WOCs), those featuring a reactive set of four multi-redox transition metals can leverage an extraordinary interplay of electronic and structural properties. These are of particular interest, owing to their close structural, and possibly functional, relationship to the oxygen evolving complex of natural photosynthesis. In this review, special attention is given to two classes of tetrametallic molecular WOCs: (i) M(4)O(4) cubane-type structures stabilized by simple organic ligands, and (ii) systems in which a tetranuclear metal core is stabilized by coordination of two polyoxometalate (POM) ligands. Recent work in this rapidly evolving field is reviewed, with particular emphasis on photocatalytic aspects. Special attention is given to studies addressing the mechanistic complexity of these systems, sometimes overlooked in the rush for oxygen evolving performance. The complementary role of molecular WOCs and their relationship with bulk oxides and heterogeneous catalysis are discussed.
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Cites
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
Proton-coupled electron transfer
Huynh, M. H. V., & Meyer, T. J. (2007) · Chemical Reviews · doi:10.1021/cr0500030 · Cited by 1,659
Leung, C.-F., Ng, S.-M., Ko, C.-C., Man, W.-L., Wu, J., Chen, L., & Lau, T.-C. (2012) · Energy & Environmental Science · doi:10.1039/c2ee21840b · Cited by 206
Cited by
Polyoxometalate-Based Cobalt–Phosphate Molecular Catalysts for Visible Light-Driven Water Oxidation
Han, X.-B., Zhang, Z.-M., Zhang, T., Li, Y.-G., Lin, W., You, W., Su, Z.-M., & Wang, E.-B. (2014) · Journal of the American Chemical Society · doi:10.1021/ja412886e · Cited by 462
Metadata
- Authors
- Sartorel, A., Bonchio, M., Campagna, S., & Scandola, F.
- Venue
- Chem. Soc. Rev.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 42
- Issue
- 6
- Pages
- 2262-2280
- ISSN
- 0306-0012 (ISSN-L)
- 1460-4744
- OpenAlex
- W2116085373
- Cited by
- 329
- References
- 3
- FWCI
- 1.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sartorel, A., Bonchio, M., Campagna, S., & Scandola, F. (2013). Tetrametallic molecular catalysts for photochemical water oxidation. Chem. Soc. Rev. https://doi.org/10.1039/c2cs35287g
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