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Superior CO2 uptake of N-doped activated carbon through hydrogen-bonding interaction
Abstract
Here we show that the introduction of N into a carbon surface facilitates the hydrogen-bonding interactions between the carbon surface and CO2 molecules, which accounts for the superior CO2 uptake of the N-doped activated carbons. This new finding challenges the long-held viewpoint that acid–base interactions between N-containing basic functional groups and acidic CO2 gas are responsible for the enhanced CO2 capture capacity of N-doped carbons.
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Citations
Cited by
Wei, J., Zhou, D., Sun, Z., Deng, Y., Xia, Y., & Zhao, D. (2013) · Advanced Functional Materials · doi:10.1002/adfm.201202764 · Cited by 931
Wang, R., Wang, P., Yan, X., Lang, J., Peng, C., & Xue, Q. (2012) · ACS Applied Materials & Interfaces · doi:10.1021/am302077c · Cited by 475
Enhanced CO2 Capture Capacity of Nitrogen-Doped Biomass-Derived Porous Carbons
Chen, J., Yang, J., Hu, G., Hu, X., Li, Z., Shen, S., Radosz, M., & Fan, M. (2016) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.5b01425 · Cited by 419
Importance of small micropores in CO 2 capture by phenolic resin-based activated carbon spheres
Wickramaratne, N. P., & Jaroniec, M. (2013) · J. Mater. Chem. A · doi:10.1039/c2ta00388k · Cited by 415
Petrovic, B., Gorbounov, M., & Masoudi Soltani, S. (2021) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2020.110751 · Cited by 381
Metadata
- Authors
- Xing, W., Liu, C., Zhou, Z., Zhang, L., Zhou, J., Zhuo, S., Yan, Z., Gao, H., Wang, G., & Qiao, S. Z.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 5
- Issue
- 6
- Pages
- 7323
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2057558267
- Cited by
- 500
- References
- 0
- FWCI
- 51.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xing, W., Liu, C., Zhou, Z., Zhang, L., Zhou, J., Zhuo, S., Yan, Z., Gao, H., Wang, G., & Qiao, S. Z. (2012). Superior CO2 uptake of N-doped activated carbon through hydrogen-bonding interaction. Energy & Environmental Science. https://doi.org/10.1039/c2ee21653a
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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