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Lithium storage in nitrogen-rich mesoporous carbon materials
Abstract
Nitrogen-rich mesoporous carbon materials were obtained by pyrolyzing gelatin between 700 and 900 °C with a nano-CaCO3 template. The mesoporous structure and the high nitrogen content endowed these materials with reversible capacities up to ca. 1200 mA h g−1. The high specific surface area and the nitrogen doping are responsible for the capacity loss in the initial cycle. FTIR and XPS studies indicate that the nitrogen in the material exists in the form of pyridinic, pyrrolic/pyridonic and graphitic nitrogen. The Raman spectroscopic analysis indicates that the structure of the mesoporous carbon becomes more disordered during discharge and is restored during recharge, a behavior similar to that in nitrogen-free hard carbon materials. The reversible structural variation of these carbon materials ensures their high cyclic reversibility.
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Cites
Chen, Y., Wang, J., Liu, H., Banis, M. N., Li, R., Sun, X., Sham, T.-K., Ye, S., & Knights, S. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp108864y · Cited by 241
Cited by
Li, Z., Xu, Z., Tan, X., Wang, H., Holt, C. M. B., Stephenson, T., Olsen, B. C., & Mitlin, D. (2013) · Energy & Environmental Science · doi:10.1039/c2ee23599d · Cited by 1,054
Wu, G., Santandreu, A., Kellogg, W., Gupta, S., Ogoke, O., Zhang, H., Wang, H.-L., & Dai, L. (2016) · Nano Energy · doi:10.1016/j.nanoen.2015.12.032 · Cited by 744
Biomass-derived porous carbon materials with sulfur and nitrogen dual-doping for energy storage
Xu, G., Han, J., Ding, B., Nie, P., Pan, J., Dou, H., Li, H., & Zhang, X. (2015) · Green Chemistry · doi:10.1039/c4gc02185a · Cited by 649
Graphitic Carbon Nanocage as a Stable and High Power Anode for Potassium‐Ion Batteries
Cao, B., Zhang, Q., Liu, H., Xu, B., Zhang, S., Zhou, T., Mao, J., Pang, W. K., Guo, Z., Li, A., et al. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201801149 · Cited by 561
Self-citationWu, K., Huang, J., Yi, J., Liu, X., Liu, Y., Wang, Y., Zhang, J., & Xia, Y. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903977 · Cited by 522
Metadata
- Authors
- Mao, Y., Duan, H., Xu, B., Zhang, L., Hu, Y., Zhao, C., Wang, Z., Chen, L., & Yang, Y.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 5
- Issue
- 7
- Pages
- 7950
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2067661850
- Cited by
- 627
- References
- 1
- FWCI
- 28.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Mao, Y., Duan, H., Xu, B., Zhang, L., Hu, Y., Zhao, C., Wang, Z., Chen, L., & Yang, Y. (2012). Lithium storage in nitrogen-rich mesoporous carbon materials. Energy & Environmental Science. https://doi.org/10.1039/c2ee21817h
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