The DOI matches its Crossref record; 30 of the 30 references it cites were found in a registry or an index.
Stability investigations of electrocatalysts on the nanoscale
Abstract
The search for more stable electrocatalyst materials for electrochemical energy conversion requires a fundamental understanding of the underlying degradation processes. Advanced characterization techniques like identical location transmission electron microscopy (IL-TEM) can provide invaluable insight into the stability of electrode materials on the nanoscale. In this review, the basic principles and the methodology of IL-TEM are described, and its capabilities are revealed by demonstrating the recent progress that has been achieved in research on the stability of fuel cell catalysts. Moreover, we provide future perspectives of the identical location approach towards implementing other electron microscopic and tomographic applications, which will help us to gain an even broader view of the degradation of electrocatalysts.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
What are batteries, fuel cells, and supercapacitors?
Winter, M., & Brodd, R. J. (2004) · Chemical Reviews · doi:10.1021/cr020730k · Cited by 7,389
Gasteiger, H. A., Kocha, S. S., Sompalli, B., & Wagner, F. T. (2005) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2004.06.021 · Cited by 4,876
Scientific Aspects of Polymer Electrolyte Fuel Cell Durability and Degradation
Borup, R., Meyers, J., Pivovar, B., Kim, Y. S., Mukundan, R., Garland, N., Myers, D., Wilson, M., Garzon, F., Wood, D., et al. (2007) · Chemical Reviews · doi:10.1021/cr050182l · Cited by 3,402
Photo-electrochemical hydrogen generation from water using solar energy. Materials-related aspects
Bak, T., Nowotny, J., Rekas, M., & Sorrell, C. C. (2002) · International Journal of Hydrogen Energy · doi:10.1016/s0360-3199(02)00022-8 · Cited by 1,546
Instability of Pt∕C Electrocatalysts in Proton Exchange Membrane Fuel Cells
Ferreira, P. J., la O’, G. J., Shao-Horn, Y., Morgan, D., Makharia, R., Kocha, S., & Gasteiger, H. A. (2005) · Journal of The Electrochemical Society · doi:10.1149/1.2050347 · Cited by 1,491
Paulus, U. A., Schmidt, T. J., Gasteiger, H. A., & Behm, R. J. (2001) · Journal of Electroanalytical Chemistry · doi:10.1016/s0022-0728(00)00407-1 · Cited by 1,427
Characterization of High‐Surface‐Area Electrocatalysts Using a Rotating Disk Electrode Configuration
Schmidt, T. J., Gasteiger, H. A., Stäb, G. D., Urban, P. M., Kolb, D. M., & Behm, R. J. (1998) · Journal of The Electrochemical Society · doi:10.1149/1.1838642 · Cited by 1,131
Recent advances in activity and durability enhancement of Pt/C catalytic cathode in PEMFC
Yu, X., & Ye, S. (2007) · Journal of Power Sources · doi:10.1016/j.jpowsour.2007.07.048 · Cited by 1,098
Instability of Supported Platinum Nanoparticles in Low-Temperature Fuel Cells
Shao-Horn, Y., Sheng, W. C., Chen, S., Ferreira, P. J., Holby, E. F., & Morgan, D. (2007) · Topics in Catalysis · doi:10.1007/s11244-007-9000-0 · Cited by 939
A review of platinum-based catalyst layer degradation in proton exchange membrane fuel cells
Zhang, S., Yuan, X.-Z., Hin, J. N. C., Wang, H., Friedrich, K. A., & Schulze, M. (2009) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.06.073 · Cited by 661
Degradation Mechanisms of Pt/C Fuel Cell Catalysts under Simulated Start–Stop Conditions
Meier, J. C., Galeano, C., Katsounaros, I., Topalov, A. A., Kostka, A., Schüth, F., & Mayrhofer, K. J. J. (2012) · ACS Catalysis · doi:10.1021/cs300024h · Cited by 586
Self-citationGraphite and carbon powders for electrochemical applications
Wissler, M. (2006) · Journal of Power Sources · doi:10.1016/j.jpowsour.2006.02.064 · Cited by 450
Fuel cell catalyst degradation on the nanoscale
Mayrhofer, K. J. J., Meier, J. C., Ashton, S. J., Wiberg, G. K. H., Kraus, F., Hanzlik, M., & Arenz, M. (2008) · Electrochemistry Communications · doi:10.1016/j.elecom.2008.05.032 · Cited by 358
Self-citation3D Imaging of Catalyst Support Corrosion in Polymer Electrolyte Fuel Cells
Schulenburg, H., Schwanitz, B., Linse, N., Scherer, G. G., Wokaun, A., Krbanjevic, J., Grothausmann, R., & Manke, I. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp203016u · Cited by 229
Yu, Y., Xin, H. L., Hovden, R., Wang, D., Rus, E. D., Mundy, J. A., Muller, D. A., & Abruña, H. D. (2012) · Nano Letters · doi:10.1021/nl203920s · Cited by 175
Mayrhofer, K. J. J., Ashton, S. J., Meier, J. C., Wiberg, G. K. H., Hanzlik, M., & Arenz, M. (2008) · Journal of Power Sources · doi:10.1016/j.jpowsour.2008.08.003 · Cited by 168
Self-citationImpact of Glass Corrosion on the Electrocatalysis on Pt Electrodes in Alkaline Electrolyte
Mayrhofer, K. J. J., Wiberg, G. K. H., & Arenz, M. (2007) · Journal of The Electrochemical Society · doi:10.1149/1.2800752 · Cited by 161
Self-citationHartl, K. G., Hanzlik, M., & Arenz, M. (2010) · Energy & Environmental Science · doi:10.1039/c0ee00248h · Cited by 155
Sheng, W., Chen, S., Vescovo, E., & Shao-Horn, Y. (2011) · Journal of The Electrochemical Society · doi:10.1149/2.009202jes · Cited by 150
Pérez-Alonso, F. J., Elkjær, C. F., Shim, S. S., Abrams, B. L., Stephens, I. E. L., & Chorkendorff, I. (2011) · Journal of Power Sources · doi:10.1016/j.jpowsour.2011.03.064 · Cited by 129
Identical-location TEM investigations of Pt/C electrocatalyst degradation at elevated temperatures
Schlögl, K., Mayrhofer, K. J. J., Hanzlik, M., & Arenz, M. (2011) · Journal of Electroanalytical Chemistry · doi:10.1016/j.jelechem.2011.09.003 · Cited by 128
Self-citationLiu, Z. Y., Zhang, J. L., Yu, P., Zhang, J. X., Makharia, R. R., More, K. L., & Stach, E. A. (2010) · Journal of The Electrochemical Society · doi:10.1149/1.3391737 · Cited by 119
The Corrosion of Carbon Black in Phosphoric Acid
Gruver, G. A. (1978) · Journal of The Electrochemical Society · doi:10.1149/1.2131280 · Cited by 73
Mayrhofer, K. J. J., Ashton, S., KREUZER, J., & Arenz, M. (2009) · International Journal of Electrochemical Science · doi:10.1016/s1452-3981(23)15133-9 · Cited by 59
Self-citationQuantitative Structural Assessment of Heterogeneous Catalysts by Electron Tomography
Grothausmann, R., Zehl, G., Manke, I., et al. (2011) · Journal of the American Chemical Society · doi:10.1021/ja2032508 · Cited by 57
Comparative IL-TEM Study Concerning the Degradation of Carbon Supported Pt-Based Electrocatalysts
Schlögl, K., Hanzlik, M., & Arenz, M. (2012) · Journal of The Electrochemical Society · doi:10.1149/2.035206jes · Cited by 54
In SituHREM Observation of Crystalline-to-Gas Transition in Nanometer-Sized Ag Particles
Lee, J.-G., Lee, J., Lee, J., Lee, J., Tanaka, T., & Mori, H. (2006) · Physical Review Letters · doi:10.1103/physrevlett.96.075504 · Cited by 53
Coarsening of Pt Nanoparticles in Proton Exchange Membrane Fuel Cells upon Potential Cycling
Shao‐Horn, Y., Ferreira, P. J., la O’, G. J., Morgan, D. D., Gasteiger, H. A., & Makharia, R. R. (2006) · ECS Transactions · doi:10.1149/1.2214553 · Cited by 51
Effect of operational potential on performance decay rate in a phosphoric acid fuel cell
Aragane, J., Urushibata, H., & Murahashi, T. (1996) · Journal of Applied Electrochemistry · doi:10.1007/bf00364064 · Cited by 49
Research works printed but not linked: 1
- Akita, 2005, J. Mater. Sci., 40, 3101, 10.1007/s10853-005-2670-8 · doi:10.1007/s10853-005-2670-8
Cited by
A metal–organic framework-derived bifunctional oxygen electrocatalyst
Xia, B. Y., Yan, Y., Li, N., Wu, H. B., Lou, X. W., & Wang, X. (2016) · Nature Energy · doi:10.1038/nenergy.2015.6 · Cited by 2,247
Design criteria for stable Pt/C fuel cell catalysts
Meier, J. C., Galeano, C., Katsounaros, I., Witte, J., Bongard, H. J., Topalov, A. A., Baldizzone, C., Mezzavilla, S., Schüth, F., & Mayrhofer, K. J. J. (2014) · Beilstein Journal of Nanotechnology · doi:10.3762/bjnano.5.5 · Cited by 559
Self-citationPei, Z., Li, H., Huang, Y., Xue, Q., Huang, Y., Zhu, M., Wang, Z., & Zhi, C. (2017) · Energy & Environmental Science · doi:10.1039/c6ee03265f · Cited by 484
Dissolution of Platinum: Limits for the Deployment of Electrochemical Energy Conversion?
Topalov, A. A., Katsounaros, I., Auinger, M., Cherevko, S., Meier, J. C., Klemm, S. O., & Mayrhofer, K. J. J. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201207256 · Cited by 428
Self-citationHuge Instability of Pt/C Catalysts in Alkaline Medium
Zadick, A., Dubau, L., Sergent, N., Berthomé, G., & Chatenet, M. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b01037 · Cited by 422
Metadata
- Authors
- Meier, J. C., Katsounaros, I., Galeano, C., Bongard, H. J., Topalov, A. A., Kostka, A., Karschin, A., Schüth, F., & Mayrhofer, K. J. J.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 5
- Issue
- 11
- Pages
- 9319
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2118401551
- Cited by
- 256
- References
- 30
- FWCI
- 6.68
- Type
- journal article
- Language
- en
- Open access
- closed
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
