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Electrodeposited Pt on three-dimensional interconnected graphene as a free-standing electrode for fuel cell application

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Maiyalagan, Thandavarayan, Dong, Xiaochen, Chen, Peng, Wang, Xin·2012·Journal of Materials Chemistry

Abstract

A three-dimensional interconnected graphene monolith was used as an electrode support for pulsed electrochemical deposition of platinum (Pt) nanoparticles. Pt nanoparticles with well-defined morphology and small size can be obtained by controlling electrodeposition potential and time. Electrochemical characterization was carried out to examine the electrocatalytic activity of this monolithic electrode towards methanol oxidation in acidic media. The results show that the carbon material surface and structure have a strong influence on the Pt particle size and morphology. Compared with the three-dimensional scaffold of carbon fibers, the three-dimensional graphene when used as a free-standing electrode support resulted in much improved catalytic activity for methanol oxidation in fuel cells due to its three-dimensionally interconnected seamless porous structure, high surface area and high conductivity.

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Metadata

Authors
Maiyalagan, T., Dong, X., Chen, P., & Wang, X.
Venue
Journal of Materials Chemistry
Published
2012
Volume
22
Issue
12
Pages
5286
ISSN
  • 0959-9428 (ISSN-L)
  • 1364-5501
OpenAlex
W1981173904
Cited by
232
References
0
FWCI
12.03
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Electrodeposited Pt on three-dimensional interconnected graphene as a free-standing electrode for fuel cell application. https://app.cochat.ai/papers/10.1039/c2jm16541d
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Maiyalagan, T., Dong, X., Chen, P., & Wang, X. (2012). Electrodeposited Pt on three-dimensional interconnected graphene as a free-standing electrode for fuel cell application. Journal of Materials Chemistry. https://doi.org/10.1039/c2jm16541d

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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.