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Structural requirements for fast lithium ion migration in Li10GeP2S12
Abstract
Dynamic lithium distribution, structural stability and ion transport mechanism in the new ultrafast ion conductor Li10GeP2S12 are clarified with the help of atomistic molecular dynamics simulations, revealing only a weak anisotropy of Li+ diffusion, and a coupling of Li+ cation diffusion to PS43− anion rotational mobility. The role of a previously overlooked Li site and the limited structural stability at elevated temperatures are discussed for the first time.
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Citations
Cites
Lithium Batteries: Status, Prospects and Future
Scrosati, B., & Garche, J. (2010) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.11.048 · Cited by 5,153
Cited by
Ong, S. P., Mo, Y., Richards, W. D., Miara, L., Lee, H. S., & Ceder, G. (2013) · Energy Environ. Sci. · doi:10.1039/c2ee23355j · Cited by 710
Zhang, Q., Cao, D., Ma, Y., Natan, A., Aurora, P., & Zhu, H. (2019) · Advanced Materials · doi:10.1002/adma.201901131 · Cited by 709
Sulfide Solid Electrolytes for Lithium Battery Applications
Lau, J., DeBlock, R. H., Butts, D. M., Ashby, D. S., Choi, C. S., & Dunn, B. S. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201800933 · Cited by 678
Li10SnP2S12: An Affordable Lithium Superionic Conductor
Bron, P., Johansson, S., Zick, K., Schmedt auf der Günne, J., Dehnen, S., & Roling, B. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407393y · Cited by 655
Computation-Accelerated Design of Materials and Interfaces for All-Solid-State Lithium-Ion Batteries
Nolan, A. M., Zhu, Y., He, X., Bai, Q., & Mo, Y. (2018) · Joule · doi:10.1016/j.joule.2018.08.017 · Cited by 398
Metadata
- Authors
- Adams, S., & Prasada Rao, R.
- Venue
- Journal of Materials Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 22
- Issue
- 16
- Pages
- 7687
- ISSN
- 0959-9428 (ISSN-L)
- 1364-5501
- OpenAlex
- W2016322040
- Cited by
- 176
- References
- 1
- FWCI
- 6.10
- Type
- journal article
- Language
- en
- Open access
- closed
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- Adams, S., & Prasada Rao, R. (2012). Structural requirements for fast lithium ion migration in Li10GeP2S12. Journal of Materials Chemistry. https://doi.org/10.1039/c2jm16688g
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
