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Cited by 30Organic Electronics and PhotovoltaicsPorphyrin and Phthalocyanine ChemistryPhotodynamic Therapy Research Studies

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Photosensitizing porphyrin–triazine compound for bulk heterojunction solar cells

Luechai, Aritat, Gasiorowski, Jacek, Petsom, Amorn, Neugebauer, Helmut, Sariciftci, Niyazi Serdar, Thamyongkit, Patchanita·2012·Journal of Materials Chemistry
DOI 10.1039/c2jm33840h
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Abstract

This report describes the synthesis of a novel porphyrin–triazine compound bearing three porphyrin macrocycles connected to each other via a triazine central unit, and investigation of its properties for possible use in bulk heterojunction solar cells (BHJ-SCs). The porphyrin macrocycles serve as light harvesting antennae, while the triazines have been widely known to be charge extracting promoters. According to cyclic voltammetric studies, the Highest Occupied Molecular Orbital (HOMO) and Lowest Unoccupied Molecular Orbital (LUMO) energy levels of the target compound were estimated to be at −5.4 and −3.5 eV versus vacuum, respectively. Photoluminescence measurements of the blended films of the porphyrin–triazine compound and phenyl-C61-butyric acid methyl ester (PCBM) or poly(3-hexylthiophene) (P3HT) indicated that the charge transfer was possible when the target porphyrin was used as an electron donor together with PCBM as an acceptor. Additionally, the surface morphology of the films with different donor : acceptor ratios was investigated by atomic force microscopy (AFM). Upon variation of the donor : acceptor weight ratio and thickness of the organic layer, the short circuit current density (JSC) of the BHJ-SCs fabricated herein improved up to approximately 2.25 mA cm−2.

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  • In the case of G1, the energy difference in the LUMOs of the donor and the acceptor is 0.7 eV; this is too high, and there might be less chance of electron-hole dissociation.

    “In the case of G1 , the energy di ff erence in the LUMOs of the donor and the acceptor is 0.7 eV; this is too high, and there might be less chance of electron -hole dissociation.”

    From Recent progress in porphyrin-based materials for organic solar cells (2018) · cites this paper as [124]

  • G1:PC61BM with a ratio of 1:10 showed a PCE of 0.5%.

    “G1 : PC61BM with a ratio of 1 : 10 showed a PCE of 0.5%.”

    From Recent progress in porphyrin-based materials for organic solar cells (2018) · cites this paper as [124]

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Cited by

Sorted by citations

Metadata

Authors
Luechai, A., Gasiorowski, J., Petsom, A., Neugebauer, H., Sariciftci, N. S., & Thamyongkit, P.
Affiliations
  • Chulalongkorn University (TH)
  • Johannes Kepler University of Linz (AT)
Corresponding author
Thamyongkit, Patchanita
ORCID
Venue
Journal of Materials Chemistry
Publisher
Royal Society of Chemistry (RSC)
Published
2012
Volume
22
Issue
43
Pages
23030
ISSN
  • 0959-9428 (ISSN-L)
  • 1364-5501
DOI
10.1039/c2jm33840h
OpenAlex
W1987090405
Cited by
30
References
2
Citations by year
2022: 1 · 2021: 2 · 2018: 2 · 2016: 5 · 2015: 8 · 2014: 9 · 2013: 3
FWCI
4.09
Type
journal article
Language
en
Open access
closed
Locations
Journal of Materials Chemistry (publishedVersion)
Topics
  • Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Electronics and Photovoltaics
  • Physical Sciences › Materials Science › Materials Chemistry › Porphyrin and Phthalocyanine Chemistry
  • Life Sciences › Biochemistry, Genetics and Molecular Biology › Cancer Research › Photodynamic Therapy Research Studies
Keywords
bulk heterojunction solar cells, organic solar cells, macrocyclic porphyrins, triazines, charge extraction, HOMO-LUMO energy levels, PCBM, poly(3-hexylthiophene), donor-acceptor blends, charge transfer, short-circuit current density, film morphology

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