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Strongly visible-light responsive plasmonic shaped AgX:Ag (X = Cl, Br) nanoparticles for reduction of CO2 to methanol
Abstract
Plasmonic shaped AgX:Ag (X = Cl, Br) nanoparticles have been synthesized by a facile and versatile glycerol-mediated solution route. The as-prepared AgX:Ag nanoparticles exhibit regular shapes, i.e., cube-tetrapod-like AgCl:Ag nanoparticles and AgBr:Ag nanoplates. Compared with the pristine AgX, AgX:Ag nanocomposites display stronger absorption in the visible region due to the surface plasmon resonance of silver nanoparticles. The calculation of bandgaps and band positions indicates the as-achieved AgX:Ag nanoparticles can be used as a class of potential photocatalyst for the reduction of CO(2). For example, reduction of CO(2) under visible light irradiation with the assistance of the anisotropic AgX:Ag nanoparticles yields as much as 100 μmol methanol in the products. Furthermore, the AgX:Ag nanoparticles can maintain its structure and activity after 3 runs of reactions. Therefore, the present route opens an avenue to acquire plasmonic photocatalysts for conversion of CO(2) into useful organic compounds.
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Cited by
Vu, N., Kaliaguine, S., & Do, T. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901825 · Cited by 445
Zhang, S., Li, J., Wang, X., Huang, Y., Zeng, M., & Xu, J. (2014) · ACS Applied Materials & Interfaces · doi:10.1021/am505528c · Cited by 432
Hsieh, Y.-C., Senanayake, S. D., Zhang, Y., Xu, W., & Polyansky, D. E. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b01235 · Cited by 396
Ong, W., Tan, L., Chai, S., Yong, S., & Mohamed, A. R. (2014) · ChemSusChem · doi:10.1002/cssc.201300924 · Cited by 339
Metadata
- Authors
- An, C., Wang, J., Jiang, W., Zhang, M., Ming, X., Wang, S., & Zhang, Q.
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 4
- Issue
- 18
- Pages
- 5646
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W2171305973
- Cited by
- 213
- References
- 0
- FWCI
- 7.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Strongly visible-light responsive plasmonic shaped AgX:Ag (X = Cl, Br) nanoparticles for reduction of CO2 to methanol. https://app.cochat.ai/papers/10.1039/c2nr31213a
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- An, C., Wang, J., Jiang, W., Zhang, M., Ming, X., Wang, S., & Zhang, Q. (2012). Strongly visible-light responsive plasmonic shaped AgX:Ag (X = Cl, Br) nanoparticles for reduction of CO2 to methanol. Nanoscale. https://doi.org/10.1039/c2nr31213a
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