The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Advanced chemical recycling of poly(ethylene terephthalate) through organocatalytic aminolysis
Abstract
We report the effective organocatalysis of the aminolytic depolymerization of waste poly(ethylene terephthalate) (PET) using 1,5,7-triazabicyclo[4.4.0]dec-5-ene (TBD) producing a broad range of crystalline terephthalamides. This diverse set of monomers possesses great potential as building blocks for high performance materials with desirable thermal and mechanical properties deriving from the terephthalic moiety and amide hydrogen bonding. Further, a computational study established mechanistic insight into self-catalyzed and organocatalyzed aminolysis of terephthalic esters, suggesting that the bifunctionality of TBD particularly concerning activation of the carbonyl group differentiates TBD from other organic bases.
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Cites
Chemical Recycling of Poly(ethylene terephthalate)
Paszun, D., & Spychaj, T. (1997) · Industrial & Engineering Chemistry Research · doi:10.1021/ie960563c · Cited by 661
Torres, N., Robin, J. J., & Boutevin, B. (2000) · European Polymer Journal · doi:10.1016/s0014-3057(99)00301-8 · Cited by 248
Horn, H. W., Jones, G. O., Wei, D. S., Fukushima, K., Lecuyer, J. M., Coady, D. J., Hedrick, J. L., & Rice, J. E. (2012) · The Journal of Physical Chemistry A · doi:10.1021/jp304212y · Cited by 97
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Cited by
Chemical recycling of waste plastics for new materials production
Rahimi, A., & García, J. M. (2017) · Nature Reviews Chemistry · doi:10.1038/s41570-017-0046 · Cited by 2,121
Chemical recycling to monomer for an ideal, circular polymer economy
Coates, G. W., & Getzler, Y. D. Y. L. (2020) · Nature Reviews Materials · doi:10.1038/s41578-020-0190-4 · Cited by 1,644
Chemically recyclable polymers: a circular economy approach to sustainability
Hong, M., & Chen, E. Y.-X. (2017) · Green Chemistry · doi:10.1039/c7gc01496a · Cited by 876
Closed-loop recycling of plastics enabled by dynamic covalent diketoenamine bonds
Christensen, P. R., Scheuermann, A. M., Loeffler, K. E., & Helms, B. A. (2019) · Nature Chemistry · doi:10.1038/s41557-019-0249-2 · Cited by 676
Expanding plastics recycling technologies: chemical aspects, technology status and challenges
Li, H., Aguirre-Villegas, H. A., Allen, R. D., Bai, X., Benson, C. H., Beckham, G. T., Bradshaw, S. L., Brown, J. L., Brown, R. C., Cecon, V. S., et al. (2022) · Green Chemistry · doi:10.1039/d2gc02588d · Cited by 616
Metadata
- Authors
- Fukushima, K., Lecuyer, J. M., Wei, D. S., Horn, H. W., Jones, G. O., Al-Megren, H. A., Alabdulrahman, A. M., Alsewailem, F. D., McNeil, M. A., Rice, J. E., & Hedrick, J. L.
- Venue
- Polym. Chem.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 4
- Issue
- 5
- Pages
- 1610-1616
- ISSN
- 1759-9954 (ISSN-L)
- 1759-9962
- OpenAlex
- W2009646475
- Cited by
- 215
- References
- 3
- FWCI
- 2.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fukushima, K., Lecuyer, J. M., Wei, D. S., Horn, H. W., Jones, G. O., Al-Megren, H. A., Alabdulrahman, A. M., Alsewailem, F. D., McNeil, M. A., Rice, J. E., & Hedrick, J. L. (2013). Advanced chemical recycling of poly(ethylene terephthalate) through organocatalytic aminolysis. Polym. Chem. https://doi.org/10.1039/c2py20793a
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